High efficiency microwave absorption (MA) materials with tunable electromagnetic (EM) features have been highly sought. However, it is still a challenge to achieve multi-bands absorption performance by simple optimizing the chemical composition of MA materials. Herein, a simple solvothermal method was used to embed magnetic Fe₃O₄ nanoclusters on MoS₂ nanosheets, in which magnetic nanoclusters were quantitatively customized. More importantly, the MA frequency and MA properties of the material are highly tailored, and multi-bands absorption is achieved. The minimum reflection loss (RL) of Fe₃O₄/MoS₂ composite reaches −87.24 dB and is about 4 times more than pure MoS₂ nanosheets. The effective absorption bandwidth reaches 5.52 GHz (≤-10 dB). These desirable properties result from the introduction of appropriate magnetic Fe₃O₄ nanoclusters, which provide optimal synergistic effect of dielectric and magnetic losses. This result provides a feasible idea for designing high efficiency MA materials with tunable EM features in the future.