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Research Article | Open Access

Highly stable self-rectifying memristor integrated arrays for simulated annealing neuromorphic computing

Jiang Bian1 Yingfang Zhu2 ( )Shaoan Yan2 ( )Yin Tang1Jiayue Guo1Gang Li2 Jiang Zhao1Qing Zhong1Qingjiang Li3Sen Liu3Rui Liu1Qilai Chen4Yongguang Xiao1Xiaojian Zhu5 ( )Qinghua Li6Minghua Tang1,7 ( )
School of Materials Science and Engineering, Xiangtan University, Xiangtan 411105, China
School of Mechanical Engineering and Mechanics, Xiangtan University, Xiangtan 411105, China
College of Electronic Science and Engineering, National University of Defense Technology, Changsha 410073, China
College of Automation and Electronic Information, Xiangtan University, Xiangtan 411105, China
CAS Key Laboratory of Magnetic Materials and Devices, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo 315201, China
Wuhan Second Ship Design and Research Institute, Wuhan 430205, China
The National Center for Applied Mathematics in Hunan, Xiangtan University, Xiangtan 411105, China
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Abstract

This work presents a high-stability self-rectifying memristor (SRM) array based on the Pt/TaOx/Ti structure, with an in-depth investigation of the performance and potential applications of the device. The device demonstrates excellent rectification and on/off ratios, along with low-power readout, multi-state storage, and multi-level switching capabilities, highlighting its practicality and adaptability. Notably, the device exhibits outstanding fluctuation suppression and exceptional uniformity. The coefficient of variation (CV) of the rectification ratio, calculated as 0.11497 at 3 V, indicates its high stability under multiple cycles and low-voltage operation, making it well-suited for large-scale integration and operational applications. Moreover, the stability of the rectification ratio further reinforces its potential as a hardware foundation for large-scale in-memory computing systems. By combining the neuromorphic characteristics of the device with a simulated annealing algorithm and optimizing the annealing temperature function, the system emulates biological neuron behavior, enabling fast and efficient image restoration tasks. Experimental results demonstrate that this approach significantly outperforms traditional algorithms in both optimization speed and repair accuracy. The present study offers a novel perspective for the design of in-memory computing hardware and showcases promising applications in neuromorphic computing and image processing.

Graphical Abstract

The 1 kb self-rectifying memristor (SRM) arrays developed in this study demonstrate superior performance in rectification ratio and on/off ratio, while featuring low-power reading, multi-state storage, and multi-level switching capabilities. Notably, these devices exhibit exceptional fluctuation suppression capability and high consistency, maintaining stable operation under repeated cycles and low-voltage conditions. Additionally, this research developed a dedicated test board for SRM arrays, integrating the neural characteristics of the device with a simulated annealing algorithm. By optimizing the annealing temperature function to mimic biological neuronal behavior more closely, the system achieves rapid and efficient image restoration. Experimental results indicate that this approach significantly surpasses conventional algorithms in both optimization speed and restoration accuracy, offering novel design paradigms for in-memory computing hardware.

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Nano Research
Article number: 94907803

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Cite this article:
Bian J, Zhu Y, Yan S, et al. Highly stable self-rectifying memristor integrated arrays for simulated annealing neuromorphic computing. Nano Research, 2026, 19(1): 94907803. https://doi.org/10.26599/NR.2025.94907803
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Received: 02 April 2025
Revised: 14 July 2025
Accepted: 15 July 2025
Published: 17 December 2025
© The Author(s) 2026. Published by Tsinghua University Press.

This is an open access article under the terms of the Creative Commons Attribution 4.0 International License (CC BY 4.0, https://creativecommons.org/licenses/by/4.0/).