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Research Article | Open Access

Carbon nanodot-based flexible and self-powered white displays

Wei Zhang§Qing Lou§Junlu Sun ( )Juan LiaoGuangsong ZhengFuhang JiaoWu ChenXiang LiJiajia MengChong-Xin ShanLin Dong ( )
Henan Key Laboratory of Diamond Optoelectronic Materials and Devices, Key Laboratory of Materials Physics, Ministry of Education, School of Physics, Zhengzhou University, Zhengzhou 450052, China

§ Wei Zhang and Qing Lou contributed equally to this work.

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Abstract

Carbon nanodots (CDs) have emerged as a promising luminescent material, showing significant potential in biological imaging, information security, and illumination displays within the internet of things (IoT). However, CDs-based electroluminescent devices, especially flexible and self-powered white displays, remain scarcely reported, which limit their applications in human-machine interactions and wearable optoelectronics in the IoT. Herein, we present a pioneering CDs-based flexible and self-powered white display system with a Commission Internationale de L’Eclairage (CIE) coordinate of (0.31, 0.39) by integrating CDs-based alternating current electroluminescent (ACEL) devices with triboelectric nanogenerators. The CDs-based white ACEL devices can be dynamically modulated from light green to white under various supplied frequencies ranging from 50 to 500 Hz. The devices also render from cold white to warm white with correlated color temperature from 9705 to 4538 K, as the concentration ratios of ZnS:Cu phosphors to CDs change from 22:2 to 22:8. Furthermore, these devices exhibit excellent flexibility and stability, maintaining over 95% of their electroluminescent intensities after 4500 cycles even under a large bending angle of 180° with a bending radius of 4.9 mm. Finally, this CDs-based flexible and self-powered white display system is worn on the human body to realize real-time illumination display powered by biomechanical energy, such as hand slapping and walking. This work provides a novel design strategy toward high-performance CD-based flexible and self-powered white displays and expands their potential applications in wearable optoelectronics for the IoT.

Graphical Abstract

Carbon nanodots (CDs)-based alternating current electroluminescent (ACEL) devices are presented for the first-time by blending high-efficient yellow-emitting CDs and ZnS:Cu phosphors as emissive layers. And self-powered CDs-based flexible white display systems are obtained by integrating with triboelectric nanogenerators (TENGs). These devices can render from cold white to warm white, with correlated color temperature ranging from 9705 to 4538 K, as the concentration ratios change from 22:2 to 22:8.

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Nano Research
Article number: 94907117

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Cite this article:
Zhang W, Lou Q, Sun J, et al. Carbon nanodot-based flexible and self-powered white displays. Nano Research, 2025, 18(2): 94907117. https://doi.org/10.26599/NR.2025.94907117
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Received: 06 September 2024
Revised: 29 October 2024
Accepted: 07 November 2024
Published: 06 January 2025
© The Author(s) 2025. Published by Tsinghua University Press.

This is an open access article under the terms of the Creative Commons Attribution 4.0 International License (CC BY 4.0, https://creativecommons.org/licenses/by/4.0/).