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Review | Open Access

Recent progress and challenges of self-healing batteries

Zhonggui Quan1Xinyi Xiu2Meng Li2Li Song1( )Xuting Jin2Zhen Zhou2 ( )
Henan Institute of Advanced Technology, Zhengzhou University, Zhengzhou 450003, China
Interdisciplinary Research Center for Sustainable Energy Science and Engineering, School of Chemical Engineering, Zhengzhou University, Zhengzhou 450001, China
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Abstract

With the exponential growth of portable electronic devices and wearable technologies, batteries are currently required to deliver not only high energy density and extended cycling performance but also enhanced safety and exceptional durability. Inspired by the self-repair mechanism observed in natural systems, a self-healing strategy shows great application potential in enabling batteries to resist external physical and chemical damage. In this review, we provide a detailed exploration of the application of self-healing materials in battery components, including electrodes, electrolytes, and encapsulation layers. We also analyze the advantages and limitations of various self-healing mechanisms, highlighting their roles in optimizing battery performance. By presenting a comprehensive synthesis of existing research, the potential pathways for advancing the development of self-healing batteries are identified, as well as the key challenges and opportunities within this field. This review aims to promote the practical integration of self-healing batteries in smart and flexible electronic devices, paving the way for safer, more reliable, and long-lasting energy storage systems.

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Energy Materials and Devices
Article number: 9370058

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Review Status: {{reviewData.commendedNum}} Commended , {{reviewData.revisionRequiredNum}} Revision Required , {{reviewData.notCommendedNum}} Not Commended Under Peer Review

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Cite this article:
Quan Z, Xiu X, Li M, et al. Recent progress and challenges of self-healing batteries. Energy Materials and Devices, 2025, 3(1): 9370058. https://doi.org/10.26599/EMD.2025.9370058

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Received: 16 January 2025
Revised: 02 March 2025
Accepted: 02 March 2025
Published: 31 March 2025
© The Author(s) 2025. Published by Tsinghua University Press.

The articles published in this open access journal are distributed under the terms of the Creative Commons Attribution 4.0 International License (http://creativecommons.org/licenses/by/4.0/), which permits use, distribution and reproduction in any medium, provided the original work is properly cited.