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Research Article

Anti-Shedding and Carbon Monoxide Catalytic Removal of Flue Gas of Structural Catalyst

Xuan ZHANG1, Yingshu LIU1, Huanyu HOU2, Wenbo BIAN1, Lijun JIANG1, Chuanzhao ZHANG3, Fangzhou SUN2, Xiong YANG1, Ziyi LI1( )
School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, China
Strategic Research Institute of HBIS Group, Shijiazhuang 050023, China
College of Health and Environment, Beijing Union University, Beijing 100023, China
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Abstract

High activity and durable structural catalysts are increasingly needed for carbon monoxide (CO) catalytic removal of industrial flue gas. A series of structural catalysts were prepared by coating polymetallic oxide catalyst on cordierite honeycomb supports. The results showed that silica sol and hot air drying could promote the powder catalyst to evenly and compactly spread on the surface of the support, and improve the anti-shedding performance and catalytic performance of the structural catalyst. The coating shedding rate of the optimized catalyst after 60 min of ultrasonic vibration was 0.97%. The catalytic efficiency of 99% CO can be achieved at 7500 h–1 space speed, 1% CO, 8% water vapour content and 110 ℃, and remains stable within 72 h. The CO catalytic efficiency can be stabilized above 86% after 720 h in actual sintering flue gas condition.

CLC number: TQ426.0;O643.0 Document code: A Article ID: 0454-5648(2022)11-2924-10

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Journal of the Chinese Ceramic Society
Pages 2924-2933

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Cite this article:
ZHANG X, LIU Y, HOU H, et al. Anti-Shedding and Carbon Monoxide Catalytic Removal of Flue Gas of Structural Catalyst. Journal of the Chinese Ceramic Society, 2022, 50(11): 2924-2933. https://doi.org/10.14062/j.issn.0454-5648.20220366

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Received: 06 May 2022
Revised: 08 June 2022
Published: 29 September 2022
© 2022 Journal of the Chinese Ceramic Society