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Research Article

Construction of flower-like MoS2 decorated on Cu doped CoZn-ZIF derived N-doped carbon as superior microwave absorber

Yun Han1,§Di Lan2,§Mengjun Han1,§Zihao Xia1Jiaxiao Zou1Zirui Jia1 ( )
College of Chemistry and Chemical Engineering, Qingdao University, Qingdao 266071, China
School of Materials Science and Engineering, Hubei University of Automotive Technology, Shiyan 442002, China

§ Yun Han, Di Lan, and Mengjun Han contributed equally to this work.

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Abstract

The rational design of composition nanostructures and morphologies of the carbon-based composites materials has a significant potential for tuning electromagnetic parameters and thereby improving their performance as electromagnetic wave (EMW) absorbers. In this work, the flower-like Cu/Co-NC/MoS2 (NC = N-doped carbon skeleton) composites were successfully prepared by employing CuCoZn-ZIF (ZIF = zeolitic imidazolate framework) as precursor with subsequent annealing and hydrothermal technique. The unique flower-like morphology and electromagnetic synergy strategy between components enable the as-obtained Cu/Co-NC/MoS2 composites to exhibit outstanding microwave absorption properties. Accordingly, the minimum reflection loss of Cu/Co-NC/MoS2 reaches −54.36 dB at 2.7 mm. When the thickness reduces to 2.2 mm, the maximum effective absorption bandwidth can be achieved as large as 6.72 GHz. This research develops useful ideas for optimizing multicomponent microwave absorbing materials.

Graphical Abstract

Cu/Co-NC/MoS2 composites with unique flower-like morphology was prepared to optimize the electromagnetic synergy strategy between components and to modulate the complex dielectric parameters of the materials, thus exhibiting outstanding microwave absorption properties.

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Nano Research
Pages 8250-8260

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Cite this article:
Han Y, Lan D, Han M, et al. Construction of flower-like MoS2 decorated on Cu doped CoZn-ZIF derived N-doped carbon as superior microwave absorber. Nano Research, 2024, 17(9): 8250-8260. https://doi.org/10.1007/s12274-024-6859-z
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Received: 06 June 2024
Revised: 26 June 2024
Accepted: 02 July 2024
Published: 23 July 2024
© Tsinghua University Press 2024