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Nano Research 2023, 16(2): 3395-3407 https://doi.org/10.1007/s12274-022-5368-1
Research Article | Issue | Published: 31 December 2022

Electrospun Fe0.64Ni0.36/MXene/CNFs nanofibrous membranes with multicomponent heterostructures as flexible electromagnetic wave absorbers

Show Author's Information Shuo Zhang1,§,  Zirui Jia2,3,§( ),  Yan Zhang1,  Guanglei Wu1( )
Institute of Materials for Energy and Environment, State Key Laboratory of Bio-fibers and Eco-textiles, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, China
College of Chemistry and Chemical Engineering, Qingdao University, Qingdao 266071, China
Weihai Innovation Institute, Qingdao University, Weihai 264200, China

§ Shuo Zhang and Zirui Jia contributed equally to this work.

Keywords:
electrospinning, nanofibers, MXene, electromagnetic wave absorption, Fe0.64Ni0.36
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FabricsNanofibers
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Zhang S, Jia Z, Zhang Y, et al. Electrospun Fe0.64Ni0.36/MXene/CNFs nanofibrous membranes with multicomponent heterostructures as flexible electromagnetic wave absorbers. Nano Research, 2023, 16(2): 3395-3407. https://doi.org/10.1007/s12274-022-5368-1
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Abstract Full text Electronic supplementary material About this article

Two-dimensional metal carbide or nitride materials (MXenes) are widely used in electromagnetic wave absorption because of their unique structure. Herein, a novel composite preparation strategy has been proposed to design dendritic nanofibers based on the electrostatic spinning methods. The multifunctional MXene nanosheets are used as the dendritic matrix, and magnetic nanoparticles are embedded in the nanosheets as magnetic loss units. Multidimensional nanocomposites have interlaced carbon fiber networks, large-scale magnetically coupled networks, and a lot of multi-heterojunction interface structures, which endow the composites with extraordinary conduction loss, magnetic loss, and polarization loss capabilities, respectively. The impedance matching and loss mechanisms of the composites are improved by optimizing the synergistic relationship between the components and building a suitable structure. The optimum reflection loss (RL) of −54.1 dB is achieved at 2.7 mm and a wide effective absorption bandwidth (EAB, RL below −10 dB) of 7.76 GHz is obtained at a small thickness of 2.1 mm for the nanocomposites. The distinctive microstructures of the nanofibrous membranes give rise to their flexibility, waterproof, and electromagnetic wave absorption performance and endow the nanofibrous membranes potential to be utilized as lightweight, efficient electromagnetic wave protective fabric in harsh environment.


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Electronic supplementary material
About this article

Electrospun Fe0.64Ni0.36/MXene/CNFs nanofibrous membranes with multicomponent heterostructures as flexible electromagnetic wave absorbers

Show Author's information Shuo Zhang1,§, Zirui Jia2,3,§( ), Yan Zhang1, Guanglei Wu1( )
Institute of Materials for Energy and Environment, State Key Laboratory of Bio-fibers and Eco-textiles, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, China
College of Chemistry and Chemical Engineering, Qingdao University, Qingdao 266071, China
Weihai Innovation Institute, Qingdao University, Weihai 264200, China

§ Shuo Zhang and Zirui Jia contributed equally to this work.

Abstract

Two-dimensional metal carbide or nitride materials (MXenes) are widely used in electromagnetic wave absorption because of their unique structure. Herein, a novel composite preparation strategy has been proposed to design dendritic nanofibers based on the electrostatic spinning methods. The multifunctional MXene nanosheets are used as the dendritic matrix, and magnetic nanoparticles are embedded in the nanosheets as magnetic loss units. Multidimensional nanocomposites have interlaced carbon fiber networks, large-scale magnetically coupled networks, and a lot of multi-heterojunction interface structures, which endow the composites with extraordinary conduction loss, magnetic loss, and polarization loss capabilities, respectively. The impedance matching and loss mechanisms of the composites are improved by optimizing the synergistic relationship between the components and building a suitable structure. The optimum reflection loss (RL) of −54.1 dB is achieved at 2.7 mm and a wide effective absorption bandwidth (EAB, RL below −10 dB) of 7.76 GHz is obtained at a small thickness of 2.1 mm for the nanocomposites. The distinctive microstructures of the nanofibrous membranes give rise to their flexibility, waterproof, and electromagnetic wave absorption performance and endow the nanofibrous membranes potential to be utilized as lightweight, efficient electromagnetic wave protective fabric in harsh environment.

Keywords: electrospinning, nanofibers, MXene, electromagnetic wave absorption, Fe0.64Ni0.36

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Publication history
Copyright
Acknowledgements

Publication history

Received: 14 October 2022
Revised: 26 November 2022
Accepted: 30 November 2022
Published: 31 December 2022
Issue date: February 2023

Copyright

© Tsinghua University Press 2022

Acknowledgements

Acknowledgements

This work is financially supported by the Natural Science Foundation of Shandong Province (No. ZR2019YQ24), Taishan Scholars and Young Experts Program of Shandong Province (No. tsqn202103057), and the Qingchuang Talents Induction Program of Shandong Higher Education Institution (Research and Innovation Team of Structural-Functional Polymer Composites).

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