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Nano Research Energy https://doi.org/10.26599/NRE.2024.9120118
Review Article | Open Access | Online first | Published: 22 March 2024

Recent advances in solid-state lithium batteries based on anode engineering

Show Author's Information Yun Zheng1,§,  Yingying Shen1,§,  Junpo Guo2,3( ),  Jianding Li4,  Jun Wang5,  De Ning6,  Yinan Liu1,  Yike Huang1,  Yuxin Tang7,  Yonghong Deng5,  He Yan2( ),  Huaiyu Shao1( )
Joint Key Laboratory of the Ministry of Education, Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, Macao SAR 999078, China
Department of Chemistry and Hong Kong Branch of Chinese National Engineering Research Center for Tissue Restoration and Reconstruction, Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, Hong Kong 999077, China
School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang 453007, China
School of Science, Huzhou University, Huzhou 313000, China
School of Innovation and Entrepreneurship, Southern University of Science and Technology, Shenzhen 518055, China
Centre for Photonics Information and Energy Materials, Shenzhen Institutes of Advanced Technology, Chinese Academy of Sciences, Shenzhen 518055, China
College of Chemical Engineering, Fuzhou University, Fuzhou 350116, China

§ Yun Zheng and Yingying Shen contributed equally to this work.

Keywords:
anode materials, solid-state batteries, Li dendrite growth, interfacial contact
Cite this article:
Zheng Y, Shen Y, Guo J, et al. Recent advances in solid-state lithium batteries based on anode engineering. Nano Research Energy, 2024, https://doi.org/10.26599/NRE.2024.9120118
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Abstract Full text About this article

Since limited energy density and intrinsic safety issues of commercial lithium-ion batteries (LIBs), solid-state batteries (SSBs) are promising candidates for next-generation energy storage systems. However, their practical applications are restricted by interfacial issues and kinetic problems, which result in energy density decay and safety failure. This review discusses the formation mechanisms of these issues from the perspective of typical solid-state electrolytes (SSEs) and provides an overview of recent advanced anode engineering for SSBs based on representative anodes including Li metal, graphite-based, and Si-based anodes, summarizing the advantages and problems of each strategy. The development of the anode-free batteries concept is demonstrated as well. Finally, recommendations are proposed for the potential directions in future research in anode engineering for SSBs.


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About this article

Recent advances in solid-state lithium batteries based on anode engineering

Show Author's information Yun Zheng1,§, Yingying Shen1,§, Junpo Guo2,3( ), Jianding Li4, Jun Wang5, De Ning6, Yinan Liu1, Yike Huang1, Yuxin Tang7, Yonghong Deng5, He Yan2( ), Huaiyu Shao1( )
Joint Key Laboratory of the Ministry of Education, Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, Macao SAR 999078, China
Department of Chemistry and Hong Kong Branch of Chinese National Engineering Research Center for Tissue Restoration and Reconstruction, Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, Hong Kong 999077, China
School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang 453007, China
School of Science, Huzhou University, Huzhou 313000, China
School of Innovation and Entrepreneurship, Southern University of Science and Technology, Shenzhen 518055, China
Centre for Photonics Information and Energy Materials, Shenzhen Institutes of Advanced Technology, Chinese Academy of Sciences, Shenzhen 518055, China
College of Chemical Engineering, Fuzhou University, Fuzhou 350116, China

§ Yun Zheng and Yingying Shen contributed equally to this work.

Abstract

Since limited energy density and intrinsic safety issues of commercial lithium-ion batteries (LIBs), solid-state batteries (SSBs) are promising candidates for next-generation energy storage systems. However, their practical applications are restricted by interfacial issues and kinetic problems, which result in energy density decay and safety failure. This review discusses the formation mechanisms of these issues from the perspective of typical solid-state electrolytes (SSEs) and provides an overview of recent advanced anode engineering for SSBs based on representative anodes including Li metal, graphite-based, and Si-based anodes, summarizing the advantages and problems of each strategy. The development of the anode-free batteries concept is demonstrated as well. Finally, recommendations are proposed for the potential directions in future research in anode engineering for SSBs.

Keywords: anode materials, solid-state batteries, Li dendrite growth, interfacial contact

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Received: 30 January 2024
Revised: 22 February 2024
Accepted: 26 February 2024
Published: 22 March 2024

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© The Author(s) 2024. Published by Tsinghua University Press.

Acknowledgements

Acknowledgements

H.S. acknowledges the Macau Science and Technology Development Fund (FDCT) for funding (FDCT-MOST joint project No. 0026/2022/AMJ, project No. 0098/2020/A2, and No. 006/2022/ALC of the Macao Centre for Research and Development in Advanced Materials (2022‒2024)), Natural Science Foundation of Guangdong Province (Grant No. 2023A1515010765), Science and Technology Planning Project of Shenzhen of China (Shenzhen-Hong Kong-Macao Category C) (Grant No. SGDX20220530111004028), Science and Technology Planning Project of Guangdong Province of China (Grant No. 2023A0505030001). Y.T. acknowledges the National Key Research and Development Program (Grant No. 2022YFE0206400).

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