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Research Article | Open Access

High-entropy perovskite oxides: An emergent type of photochromic oxides with fast response for handwriting display

Xiangyu Wang, Tong Wei( ), Yingqiu Xu, Liwei Wu, Yingdong Han, Jiao Cui
College of Science, Civil Aviation University of China, Tianjin 300300, China
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Abstract

Stimulus-responsive materials are fundamental to the broad and ever-growing field of intelligence research, which bridge intelligent systems with the Internet of Things (IoT) in future lifestyles. Among these materials, writable materials have received great interest; however, carbonization and irreversible writing processes are generally inevitable for extensively investigated organic compounds. Photochromism is a potential mode of composing information. Nevertheless, inorganic materials usually exhibit weak photochromic effects. Here, a novel strategy of designing high-entropy perovskite (HEP) oxides is put forward to develop a new inorganic photochromic system with satisfying performance. A series of HEP oxides are synthesized for the first time. Benefiting from excellent photochromic features, real-time information encoding was achieved. The mechanism-related photochromism is also discussed. Distinct from the previous works, it is believed that the present photochromic-based HEP oxides provide a new and manyfold research space for the future development of conventional writable materials and the disclosing of unprecedented properties and phenomena.

Keywords

stimulus-responsive materialsinorganic materialshigh-entropy perovskite (HEP) oxidesphotochromism

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References

[1]
Stoyanova M, Nikoloudakis Y, Panagiotakis S, et al. A survey on the Internet of Things (IoT) forensics: Challenges, approaches, and open issues. IEEE Commun Surv Tut 2020, 22: 1191–1221.
Crossref Google Scholar
[2]
Shafique K, Khawaja BA, Sabir F, et al. Internet of Things (IoT) for next-generation smart systems: A review of current challenges, future trends and prospects for emerging 5G-IoT scenarios. IEEE Access 2020, 8: 23022–23040.
Crossref Google Scholar
[3]
Pan KW, Fan YY, Leng T, et al. Sustainable production of highly conductive multilayer graphene ink for wireless connectivity and IoT applications. Nat Commun 2018, 9: 5197.
Crossref Google Scholar
[4]
Tarancón A. Powering the IoT revolution with heat. Nat Electron 2019, 2: 270–271.
Crossref Google Scholar
[5]
Shi W, Guo YL, Liu YQ. When flexible organic field-effect transistors meet biomimetics: A prospective view of the Internet of Things. Adv Mater 2020, 32: 1901493.
Crossref Google Scholar
[6]
Liu JZ, Li XK, Yang X, et al. Recent advances in self-healable intelligent materials enabled by supramolecular crosslinking design. Adv Intell Syst 2021, 3: 2000183.
Crossref Google Scholar
[7]
Awasthi AK, Li JH, Koh L, et al. Circular economy and electronic waste. Nat Electron 2019, 2: 86–89.
Crossref Google Scholar
[8]
Lei T, Guan M, Liu J, et al. Biocompatible and totally disintegrable semiconducting polymer for ultrathin and ultralightweight transient electronics. PNAS 2017, 114: 5107–5112.
Crossref Google Scholar
[9]
Wang Q, Yang J, Altstädt V, et al. SusMat: Materials innovation for sustainable development. SusMat 2021, 1: 2–3.
Crossref Google Scholar
[10]
Teng L, Ye SC, Handschuh-Wang S, et al. Liquid metal-based transient circuits for flexible and recyclable electronics. Adv Funct Mater 2019, 29: 1808739.
Crossref Google Scholar
[11]
Wang H, Liu HC, Cao ZX, et al. Room-temperature autonomous self-healing glassy polymers with hyperbranched structure. PNAS 2020, 117: 11299–11305.
Crossref Google Scholar
[12]
Zhang CH, Li YJ, Kang WB, et al. Current advances and future perspectives of additive manufacturing for functional polymeric materials and devices. SusMat 2021, 1: 127–147.
Crossref Google Scholar
[13]
Chen C, Wang X, Wang Y, et al. Additive manufacturing of piezoelectric materials. Adv Funct Mater 2020, 30: 2005141.
Crossref Google Scholar
[14]
Van Ewijk S, Stegemann JA, Ekins P. Limited climate benefits of global recycling of pulp and paper. Nat Sustain 2020, 4: 180–187.
Crossref Google Scholar
[15]
Chen C, Zhao XK, Chen YJ, et al. Reversible writing/re-writing polymeric paper in multiple environments. Adv Funct Mater 2021, 31: 2104784.
Crossref Google Scholar
[16]
Liu J, Chen Z, Chen YJ, et al. Ionic conductive organohydrogels with dynamic pattern behavior and multi-environmental stability. Adv Funct Mater 2021, 31: 2101464.
Crossref Google Scholar
[17]
Ma Y, Yu YX, Li JG, et al. Stimuli-responsive photofunctional materials for green and security printing. InfoMat 2021, 3: 82–100.
Crossref Google Scholar
[18]
Yamamoto S, Furuya H, Tsutsui K, et al. In situ observation of thermochromic behavior of binary mixtures of phenolic long-chain molecules and fluoran dye for rewritable paper application. Cryst Growth Des 2008, 8: 2256–2263.
Crossref Google Scholar
[19]
Roth PJ, Lowe AB. Stimulus-responsive polymers. Polym Chem 2017, 8: 10–11.
Crossref Google Scholar
[20]
Nagarkar SS, Desai AV, Ghosh SK. Stimulus-responsive metal–organic frameworks. Chem-Asian J 2014, 9: 2358– 2376.
Crossref Google Scholar
[21]
Ding YC, So B, Cao JK, et al. Ultrasound-induced mechanoluminescence and optical thermometry toward stimulus-responsive materials with simultaneous trigger response and read-out functions. Adv Sci 2022, 9: 2201631.
Crossref Google Scholar
[22]
Wei T, Jia B, Shen LH, et al. A new class of upconversion luminescence tuning materials based on non-photochromic reaction: Er3+-activated Ba0.7Sr0.3Nb2O6 ferroelectrics. Acta Mater 2021, 205: 116557.
Crossref Google Scholar
[23]
Wei T, Shi YC, Wang XY, et al. Realization of multiple luminescence manipulation in tungsten bronze oxides based on photochromism toward real-time, reversible, and fast processes. Inorg Chem Front 2023, 10: 2653–2664.
Crossref Google Scholar
[24]
Wang W, Han B, Zhang Y, et al. Laser-induced graphene tapes as origami and stick-on labels for photothermal manipulation via Marangoni effect. Adv Funct Mater 2021, 31: 2006179.
Crossref Google Scholar
[25]
Del Pozo M, Delaney C, Bastiaansen CWM, et al. Direct laser writing of four-dimensional structural color microactuators using a photonic photoresist. ACS Nano 2020, 14: 9832–9839.
Crossref Google Scholar
[26]
You R, Liu YQ, Hao YL, et al. Laser fabrication of graphene-based flexible electronics. Adv Mater 2020, 32: 1901981.
Crossref Google Scholar
[27]
Le XX, Shang H, Yan HZ, et al. A urease-containing fluorescent hydrogel for transient information storage. Angew Chem Int Ed 2021, 60: 3640–3646.
Crossref Google Scholar
[28]
Kayani ABA, Kuriakose S, Monshipouri M, et al. UV photochromism in transition metal oxides and hybrid materials. Small 2021, 17: 2100621.
Crossref Google Scholar
[29]
Badour Y, Jubera V, Andron I, et al. Photochromism in inorganic crystallised compounds. Opt Mater X 2021, 12: 100110.
Crossref Google Scholar
[30]
Wang SF, Fan WR, Liu ZC, et al. Advances on tungsten oxide based photochromic materials: Strategies to improve their photochromic properties. J Mater Chem C 2018, 6: 191–212.
Crossref Google Scholar
[31]
He T, Yao JN. Photochromism in transition-metal oxides. Res Chem Intermediat 2004, 30: 459–488.
Crossref Google Scholar
[32]
Yeh JW, Chen SK, Lin SJ, et al. Nanostructured high-entropy alloys with multiple principal elements: Novel alloy design concepts and outcomes. Adv Eng Mater 2004, 6: 299–303.
Crossref Google Scholar
[33]
Rost CM, Sachet E, Borman T, et al. Entropy-stabilized oxides. Nat Commun 2015, 6: 8485.
Crossref Google Scholar
[34]
Liu JX, Shen XQ, Wu Y, et al. Mechanical properties of hot-pressed high-entropy diboride-based ceramics. J Adv Ceram 2020, 9: 503–510.
Crossref Google Scholar
[35]
Zhu JT, Wei MY, Xu J, et al. Influence of order–disorder transition on the mechanical and thermophysical properties of A2B2O7 high-entropy ceramics. J Adv Ceram 2022, 11: 1222–1234.
Crossref Google Scholar
[36]
Zheng YP, Zou MC, Zhang WY, et al. Electrical and thermal transport behaviours of high-entropy perovskite thermoelectric oxides. J Adv Ceram 2021, 10: 377–384.
Crossref Google Scholar
[37]
Chen L, Li BH, Guo J, et al. High-entropy perovskite RETa3O9 ceramics for high-temperature environmental/thermal barrier coatings. J Adv Ceram 2022, 11: 556–569.
Crossref Google Scholar
[38]
Xiang HM, Xing Y, Dai FZ, et al. High-entropy ceramics: Present status, challenges, and a look forward. J Adv Ceram 2021, 10: 385–441.
Crossref Google Scholar
[39]
Zhang Z, Guo LJ, Sun HQ, et al. Rare earth orthoniobate photochromics with self-activated upconversion emissions for high-performance optical storage applications. J Mater Chem C 2021, 9: 13841–13850.
Crossref Google Scholar
[40]
Zhao HP, Cun YK, Bai X, et al. Entirely reversible photochromic glass with high coloration and luminescence contrast for 3D optical storage. ACS Energy Lett 2022, 7: 2060–2069.
Crossref Google Scholar
[41]
Yang ZT, Du JR, Martin LIDJ, et al. Highly responsive photochromic ceramics for high-contrast rewritable information displays. Laser Photonics Rev 2021, 15: 2000525.
Crossref Google Scholar
[42]
Tang W, Zuo CD, Ma CY, et al. Rapid high-contrast reversible coloration of Ba3MgSi2O8:Pr3+ photochromic materials for rewritable light-printing. J Mater Chem C 2022, 10: 18375–18384.
Crossref Google Scholar
[43]
Jin YH, Lv Y, Wang CL, et al. Design and control of the coloration degree for photochromic Sr3GdNa(PO4)3F:Eu2+ via traps modulation by Ln3+ (Ln = Y, La–Sm, Tb–Lu) co-doping. Sensor Actuat B-Chem 2017, 245: 256–262.
Crossref Google Scholar
[44]
Zhou Y, Wang P, Lin JF, et al. High-contrast photochromic Eu-doped K0.5Na0.5NbO3 ceramics with prominent pellucidity. Dalton T 2021, 50: 4914–4922.
Crossref Google Scholar
[45]
Gong J, Du P, Li WP, et al. The enhancement of photochromism and luminescence modulation properties of ferroelectric ceramics via chemical and physical strategies. Laser Photonics Rev 2022, 16: 2200170.
Crossref Google Scholar
[46]
Yang FM, Jia B, Wei T, et al. Reversible regulation of upconversion luminescence in new photochromic ferroelectric materials: Bi4−xErxTi3O12 ceramics. Inorg Chem Front 2019, 6: 2756–2766.
Crossref Google Scholar
[47]
Shannon RD. Revised effective ionic radii and systematic studies of interatomic distances in halides and chalcogenides. Acta Crystallogr A 1976, 32: 751–767.
Crossref Google Scholar
[48]
Liu ZY, Xu SC, Li T, et al. Microstructure and ferroelectric properties of high-entropy perovskite oxides with A-site disorder. Ceram Int 2021, 47: 33039–33046.
Crossref Google Scholar
[49]
Ye BL, Wen TQ, Huang KH, et al. First-principles study, fabrication, and characterization of (Hf0.2Zr0.2Ta0.2Nb0.2Ti0.2)C high-entropy ceramic. J Am Ceram Soc 2019, 102: 4344– 4352.
Crossref Google Scholar
[50]
Jiang SC, Hu T, Gild J, et al. A new class of high-entropy perovskite oxides. Scripta Mater 2018, 142: 116–120.
Crossref Google Scholar
[51]
Liu J, Ren K, Ma CY, et al. Dielectric and energy storage properties of flash-sintered high-entropy (Bi0.2Na0.2K0.2Ba0.2Ca0.2)TiO3 ceramic. Ceram Int 2020, 46: 20576–20581.
Crossref Google Scholar
[52]
Zhou SY, Pu YP, Zhang QW, et al. Microstructure and dielectric properties of high entropy Ba(Zr0.2Ti0.2Sn0.2Hf0.2Me0.2)O3 perovskite oxides. Ceram Int 2020, 46: 7430–7437.
Crossref Google Scholar
[53]
Zhang Y, Zuo TT, Tang Z, et al. Microstructures and properties of high-entropy alloys. Prog Mater Sci 2014, 61: 1–93.
Crossref Google Scholar
[54]
Lin C, Wang HJ, Wang P, et al. Smart white lighting and multi-mode optical modulations via photochromism in Dy-doped KNN-based transparent ceramics. J Am Ceram Soc 2021, 104: 903–916.
Crossref Google Scholar
[55]
Li KX, Luo LH, Zhang YY, et al. The upconversion luminescence modulation and its enhancement in Er3+-doped Na0.5Bi0.5TiO3 based on photochromic reaction. J Am Ceram Soc 2018, 101: 5640–5650.
Crossref Google Scholar
[56]
Li KX, Luo LH, Zhang YY, et al. Tunable luminescence contrast in photochromic ceramics (1−x)Na0.5Bi0.5TiO3–xNa0.5K0.5NbO3:0.002Er by an electric field poling. ACS Appl Mater Interfaces 2018, 10: 41525–41534.
Crossref Google Scholar
[57]
Chai QZ, Zhao XM, Chao XL, et al. Enhanced transmittance and piezoelectricity of transparent K0.5Na0.5NbO3 ceramics with Ca(Zn1/3Nb2/3)O3 additives. RSC Adv 2017, 7: 28428–28437.
Crossref Google Scholar
[58]
Tang W, Zuo CD, Ma CY, et al. Designing photochromic materials with high photochromic contrast and large luminescence modulation for hand-rewritable information displays and dual-mode optical storage. Chem Eng J 2022, 435: 134670.
Crossref Google Scholar
[59]
Yang ZT, Du JR, Martin LIDJ, et al. Designing photochromic materials with large luminescence modulation and strong photochromic efficiency for dual-mode rewritable optical storage. Adv Opt Mater 2021, 9: 2100669.
Crossref Google Scholar
[60]
Hu Z, Huang XJ, Yang ZW, et al. Reversible 3D optical data storage and information encryption in photo-modulated transparent glass medium. Light-Sci Appl 2021, 10: 140.
Crossref Google Scholar
[61]
Ren YT, Yang ZW, Wang YH, et al. Reversible multiplexing for optical information recording, erasing, and reading-out in photochromic BaMgSiO4:Bi3+ luminescence ceramics. Sci China Mater 2020, 63: 582–592.
Crossref Google Scholar
[62]
Bai X, Yang ZW, Zhan YH, et al. Novel strategy for designing photochromic ceramic: Reversible upconversion luminescence modification and optical information storage application in the PbWO4:Yb3+,Er3+ photochromic ceramic. ACS Appl Mater Interfaces 2020, 12: 21936–21943.
Crossref Google Scholar
[63]
Joost U, Šutka A, Oja M, et al. Reversible photodoping of TiO2 nanoparticles for photochromic applications. Chem Mater 2018, 30: 8968–8974.
Crossref Google Scholar
[64]
Wei T, Jia B, Shen LH, et al. Reversible upconversion modulation in new photochromic SrBi2Nb2O9 based ceramics for optical storage and anti-counterfeiting applications. J Eur Ceram Soc 2020, 40: 4153–4163.
Crossref Google Scholar
[65]
Wei T, Shi YC, Wang XY, et al. Engineering luminescence switching and photochromic performance in tungsten bronze oxides for handwriting display based on variable valence ion strategy. Ceram Int 2023, 49: 5788–5798.
Crossref Google Scholar
[66]
Zhang P, Zheng ZZ, Wu L, et al. Self-reduction-related defects, long afterglow, and mechanoluminescence in centrosymmetric Li2ZnGeO4:Mn2+. Inorg Chem 2021, 60: 18432–18441.
Crossref Google Scholar
Journal of Advanced Ceramics
Volume 12 Issue 7,
July 2023
Pages 1371-1388
DOI: 10.26599/JAC.2023.9220761
Cite this article:
Wang X, Wei T, Xu Y, et al. High-entropy perovskite oxides: An emergent type of photochromic oxides with fast response for handwriting display. Journal of Advanced Ceramics, 2023, 12(7): 1371-1388. https://doi.org/10.26599/JAC.2023.9220761

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Received: 10 March 2023
Revised: 15 April 2023
Accepted: 27 April 2023
Published: 21 June 2023
© The Author(s) 2023.

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