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Research Article | Open Access | Just Accepted

Investigation of the influence of substrate hardness on the tribological performance of graphene oxide solid lubricant coatings

Yuzhen LiuHui Chen( )Wenli WangKai LeGuoqing WangYong LuoXiaoming GaoXu ZhaoXingnan LiuShusheng Xu( )Dae-Eun KimWeimin Liu

a State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, China

b Shandong Laboratory of Advanced Materials and Green Manufacturing at Yantai, Yantai 264000, China

c School of Materials Science and Engineering, China University of Mining and Technology, Xuzhou 221116, China

d Department of Mechanical Engineering, Yonsei University, Seoul 03722, Republic of Korea

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Abstract

This study explores the impact of substrate hardness on the tribological properties of graphene oxide (GO) solid lubricant coatings on NiP alloy layers coated Q235 steel. Through the adjustment of electroless plating parameters, NiP alloy layers with varying hardness levels were produced to investigate their effect on the wear resistance and friction performance of GO coatings. The methodology included substrate preparation, electroless NiP alloy plating, electrophoresis deposition of GO, and detailed analysis of the structural, mechanical, and tribological characteristics of the coatings. The findings underscore the crucial role of substrate hardness in the tribological efficiency of GO coatings. A specific hardness level emerged as optimal, significantly enhancing the distribution and effectiveness of the GO tribofilm. This uniform and continuous tribofilm presence led to notable improvements in wear resistance and a reduction in friction coefficients. Moreover, this optimal hardness ensured continuous lubrication and superior load-bearing capabilities, substantially prolonging the lifespan of the coatings. The substrates with either too high or too low hardness levels were observed to hinder the maintenance of a consistent tribofilm, thereby negatively impacting the tribological performance of the coating. Conclusively, this research highlights the significance of achieving an optimal substrate hardness to enhance the tribological performance of solid lubricant coatings. By optimizing the balance between substrate hardness and the integrity of the tribofilm, the study paves the way for developing more efficient, durable, and environmentally sustainable mechanical components, offering new insights into tribological science and materials engineering.

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Cite this article:
Liu Y, Chen H, Wang W, et al. Investigation of the influence of substrate hardness on the tribological performance of graphene oxide solid lubricant coatings. Friction, 2025, https://doi.org/10.26599/FRICT.2025.9441085

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Available online: 28 February 2025

© The author(s) 2025.

The articles published in this open access journal are distributed under the terms of the Creative Commons Attribution 4.0 International License (http://creativecommons.org/licenses/by/4.0/).

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