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Research Article | Open Access

Techno-economic analysis of hydrogen-driven calcium looping process for flue gas decarbonization

Dongliang Zhang1, Hanke Li1,2 ( ), Qiangqiang Wu1, Guangxing Yang3, Hao-Fan Wang1, Yonghai Cao1, Hongjuan Wang1, Siyu Yang1 ( ), Hao Yu1 ( )
School of Chemistry and Chemical Engineering, Guangdong Provincial Key Lab of Green Chemical Product Technology, South China University of Technology, Guangzhou 510641, China
National Reference Laboratory for Food Contact Material (Guangdong), Guangzhou Customs Technology Center, Guangzhou 510075, China
School of Chemistry and Chemical Engineering, Guangzhou University, Guangzhou 510006, China
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Graphical Abstract

From a perspective of short to medium term, coke oven gas stands out as the least expensive option of alternative hydrogen source and is indeed feasible to be operated at an industrial scale for the proposed hydrogen-driven calcium looping (CaL) process, while wind-photovoltaic to hydrogen is not, unless the supportive or subsidizing programs are issued by the government or 2.15 USD per Nm3 CH4 of CH4 price.

Abstract

A techno-economic analysis was performed for a hydrogen-driven calcium looping (CaL) process capable of capturing 5 × 104–7 × 104 metric tons of CO2 per year from flue gas. The study investigated the use of coke oven gas (COG) and wind-photovoltaic to hydrogen (WPTH) as hydrogen sources. With COG as the hydrogen source, the CaL process yielded an annual production of 1.49 × 108 Nm3 CH4, an energy efficiency of 84.77%, and a payback period of 5.49 years. Conversely, using WPTH as the hydrogen source resulted in a lower annual CH4 output of 3.9 × 107 Nm3, a reduced energy efficiency of 65.04%, and annual losses of 62.10 million USD. In the near to mid-term, the hydrogen-driven CaL process enabled by COG is practically viable for industrial-scale operation. Using WPTH as the hydrogen source provides some improvements in certain aspects but drawbacks in others compared to COG. However, the considerably higher cost of producing green hydrogen remains a substantial hindrance to the process’s economic feasibility.

Keywords

calcium loopingcarbon capturehydrogen-drivenprocess integrationtechno-economic analysis

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Carbon Future
Volume 1 Issue 4,
December 2024
Article number: 9200023
DOI: 10.26599/CF.2024.9200023
Cite this article:
Zhang D, Li H, Wu Q, et al. Techno-economic analysis of hydrogen-driven calcium looping process for flue gas decarbonization. Carbon Future, 2024, 1(4): 9200023. https://doi.org/10.26599/CF.2024.9200023

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Received: 01 October 2024
Revised: 14 November 2024
Accepted: 15 November 2024
Published: 13 December 2024
© The Author(s) 2024.

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