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Friction force microscopy (FFM) explores the interaction in a sliding contact on the nanoscale, providing information on the frictional dynamics and lateral contact stiffness with lattice resolution. Recent FFM measurements on a NaCl crystal immersed in liquid (ethanol) surroundings displayed an increase of the effective contact stiffness, Keff, with the applied load, differently from similar measurements performed under ultra-high vacuum (UHV) conditions, where Keff showed negligible load dependency. Additionally, under UHV conditions multiple slip length friction with increasing load was reported, while in ethanol surroundings only single (lattice unit length) slips were observed. Our current understanding of this behavior relates the transition from single jumps to multiple jumps dynamics to the normal load (manifested through the amplitude of the interaction potential at the contact, U0) and to the damping of the system. Here we have incorporated the effect of the load dependency on both U0 and Keff within Prandtl‒Tomlinson based simulations, accompanied by variations in the damping coefficient of the system. Introducing the experimentally observed load dependency to Keff resulted indeed in single slip jumps at critical damping, while multiple slip jumps were obtained at constant Keff. The average slip length increased with the normal load, particularly when the system became underdamped. Our work provides a glimpse on the relation between the characteristic observables in atomic-scale sliding friction (maximal slip forces, stiffness, and slip dynamics) with respect to their governing parameters (corrugation energy, effective stiffness, and damping). While common understanding in nanotribology relates the effect of surrounding media mainly to the interaction potential at the contact, here we show that the media can also greatly affect the elastic interaction, and consequently play an important role on the transition from single to multiple stick-slip.


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Surroundings affect slip length dynamics in nanoscale friction through contact stiffness and damping

Show Author's information Simona SKURATOVSKY1Liron AGMON1Enrico GNECCO2Ronen BERKOVICH1,3( )
Department of Chemical Engineering, Ben-Gurion University of the Negev, Beer-Sheva 8410501, Israel
Marian Smoluchowski Institute of Physics, Jagiellonian University, Lojasiewicza 11, Krakow 30-348, Poland
Ilze Katz Institute for Nanoscience and Technology, Ben-Gurion University of the Negev, Beer-Sheva 8410501, Israel

Abstract

Friction force microscopy (FFM) explores the interaction in a sliding contact on the nanoscale, providing information on the frictional dynamics and lateral contact stiffness with lattice resolution. Recent FFM measurements on a NaCl crystal immersed in liquid (ethanol) surroundings displayed an increase of the effective contact stiffness, Keff, with the applied load, differently from similar measurements performed under ultra-high vacuum (UHV) conditions, where Keff showed negligible load dependency. Additionally, under UHV conditions multiple slip length friction with increasing load was reported, while in ethanol surroundings only single (lattice unit length) slips were observed. Our current understanding of this behavior relates the transition from single jumps to multiple jumps dynamics to the normal load (manifested through the amplitude of the interaction potential at the contact, U0) and to the damping of the system. Here we have incorporated the effect of the load dependency on both U0 and Keff within Prandtl‒Tomlinson based simulations, accompanied by variations in the damping coefficient of the system. Introducing the experimentally observed load dependency to Keff resulted indeed in single slip jumps at critical damping, while multiple slip jumps were obtained at constant Keff. The average slip length increased with the normal load, particularly when the system became underdamped. Our work provides a glimpse on the relation between the characteristic observables in atomic-scale sliding friction (maximal slip forces, stiffness, and slip dynamics) with respect to their governing parameters (corrugation energy, effective stiffness, and damping). While common understanding in nanotribology relates the effect of surrounding media mainly to the interaction potential at the contact, here we show that the media can also greatly affect the elastic interaction, and consequently play an important role on the transition from single to multiple stick-slip.

Keywords: nanoscale friction, friction force microscopy (FFM), multiple jumps, Prandtl‒Tomlinson model, effective stiffness, damping

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Publication history

Received: 19 July 2021
Revised: 04 September 2021
Accepted: 12 December 2021
Published: 04 May 2022
Issue date: February 2023

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© The author(s) 2021.

Acknowledgements

R.B. and E.G are grateful for the generous financial support of Deutsche Forschungsgemeinschaft (No. DFG GN 92/16-1).

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