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Research Article | Open Access

Vector analysis of electric-field-induced antiparallel magnetic domain evolution in ferromagnetic/ferroelectric heterostructures

Xinger ZHAOaZhongqiang HUa( )Jingen WUaTing FANGaYaojin LIaYuxin CHENGaYifan ZHAOaMengmeng GUANaDan XIANb,cChenying WANGb,cQi MAOb,cBin PENGaRen-Ci PENGaZiyao ZHOUaZhiguang WANGaZhuang-De JIANGb,cMing LIUa
Electronic Materials Research Laboratory, Key Laboratory of the Ministry of Education & International Center for Dielectric Research, School of Electronic Science and Engineering, State Key Laboratory for Mechanical Behavior of Materials, Xi’an Jiaotong University, Xi’an 710049, China
Collaborative Innovation Center of High-End Manufacturing Equipment, Xi’an Jiaotong University, Xi’an 710049, China
International Joint Laboratory for Micro/Nano Manufacturing and Measurement Technology, Xi’an Jiaotong University, Xi’an 710049, China
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Electric field (E-field) control of magnetism based on magnetoelectric coupling is one of the promising approaches for manipulating the magnetization with low power consumption. The evolution of magnetic domains under in-situ E-fields is significant for the practical applications in integrated micro/nano devices. Here, we report the vector analysis of the E-field-driven antiparallel magnetic domain evolution in FeCoSiB/PMN-PT(011) multiferroic heterostructures via in-situ quantitative magneto-optical Kerr microscope. It is demonstrated that the magnetic domains can be switched to both the 0° and 180° easy directions at the same time by E-fields, resulting in antiparallel magnetization distribution in ferromagnetic/ferroelectric heterostructures. This antiparallel magnetic domain evolution is attributed to energy minimization with the uniaxial strains by E-fields which can induce the rotation of domains no more than 90°. Moreover, domains can be driven along only one or both easy axis directions by reasonably selecting the initial magnetic domain distribution. The vector analysis of magnetic domain evolution can provide visual insights into the strain-mediated magnetoelectric effect, and promote the fundamental understanding of electrical regulation of magnetism.

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Yang SH, Ryu KS, Parkin S. Domain-wall velocities of up to 750 m·s-1 driven by exchange-coupling torque in synthetic antiferromagnets. Nat Nanotechnol 2015, 10: 221-226.
Parkin SSP, Hayashi M, Thomas L. Magnetic domain-wall racetrack memory. Science 2008, 320: 190-194.
Beach GSD, Knutson C, Nistor C, et al. Nonlinear domain- wall velocity enhancement by spin-polarized electric current. Phys Rev Lett 2006, 97: 057203.
Emori S, Bauer U, Ahn SM, et al. Current-driven dynamics of chiral ferromagnetic domain walls. Nat Mater 2013, 12: 611-616.
Miron IM, Moore T, Szambolics H, et al. Fast current- induced domain-wall motion controlled by the Rashba effect. Nat Mater 2011, 10: 419-423.
Moore TA, Miron IM, Gaudin G, et al. High domain wall velocities induced by current in ultrathin Pt/Co/AlOx wires with perpendicular magnetic anisotropy. Appl Phys Lett 2008, 93: 262504.
Matsukura F, Tokura Y, Ohno H. Control of magnetism by electric fields. Nat Nanotechnol 2015, 10: 209-220.
Spaldin NA, Ramesh R. Advances in magnetoelectric multiferroics. Nat Mater 2019, 18: 203-212.
Song C, Cui B, Li F, et al. Recent progress in voltage control of magnetism: Materials, mechanisms, and performance. Prog Mater Sci 2017, 87: 33-82.
Peng B, Zhou ZY, Nan TX, et al. Deterministic switching of perpendicular magnetic anisotropy by voltage control of spin reorientation transition in (Co/Pt)3/Pb(Mg1/3Nb2/3)O3- PbTiO3 multiferroic heterostructures. ACS Nano 2017, 11: 4337-4345.
Wu T, Bur A, Zhao P, et al. Giant electric-field-induced reversible and permanent magnetization reorientation on magnetoelectric Ni/(011) [Pb(Mg1/3Nb2/3)O3](1-x)-[PbTiO3]x heterostructure. Appl Phys Lett 2011, 98: 012504.
He X, Wang Y, Wu N, et al. Robust isothermal electric control of exchange bias at room temperature. Nat Mater 2010, 9: 579-585.
Chen A, Zhao Y, Li P, et al. Angular dependence of exchange bias and magnetization reversal controlled by electric-field-induced competing anisotropies. Adv Mater 2016, 28: 363-369.
Pantel D, Goetze S, Hesse D, et al. Reversible electrical switching of spin polarization in multiferroic tunnel junctions. Nat Mater 2012, 11: 289-293.
Chen A, Wen Y, Fang B, et al. Giant nonvolatile manipulation of magnetoresistance in magnetic tunnel junctions by electric fields via magnetoelectric coupling. Nat Commun 2019, 10: 243.
El-Ghazaly A, Evans JT, Sato N, et al. Electrically tunable integrated thin-film magnetoelectric resonators. Adv Mater Technol 2017, 2: 1700062.
Wang X, Yang Q, Wang L, et al. E-field control of the RKKY interaction in FeCoB/Ru/FeCoB/PMN-PT (011) multiferroic heterostructures. Adv Mater 2018, 30: 1803612.
Lei N, Devolder T, Agnus G, et al. Strain-controlled magnetic domain wall propagation in hybrid piezoelectric/ ferromagnetic structures. Nat Commun 2013, 4: 1378.
Kakizakai H, Ando F, Koyama T, et al. Switching local magnetization by electric-field-induced domain wall motion. Appl Phys Express 2016, 9: 063004.
Li P, Zhao Y, Zhang S, et al. Spatially resolved ferroelectric domain-switching-controlled magnetism in Co40Fe40B20/ Pb(Mg1/3Nb2/3)0.7Ti0.3O3 multiferroic heterostructure. ACS Appl Mater Interfaces 2017, 9: 2642-2649.
Ghidini M, Mansell R, Maccherozzi F, et al. Shear-strain- mediated magnetoelectric effects revealed by imaging. Nat Mater 2019, 18: 840-845.
Franke KJA, van de Wiele B, Shirahata Y, et al. Reversible electric-field-driven magnetic domain-wall motion. Phys Rev X 2015, 5: 011010.
Lahtinen THE, Franke KJA, van Dijken S. Electric-field control of magnetic domain wall motion and local magnetization reversal. Sci Rep 2012, 2: 258.
Chiba D, Kawaguchi M, Fukami S, et al. Electric-field control of magnetic domain-wall velocity in ultrathin cobalt with perpendicular magnetization. Nat Commun 2012, 3: 888.
De Ranieri E, Roy PE, Fang D, et al. Piezoelectric control of the mobility of a domain wall driven by adiabatic and non-adiabatic torques. Nat Mater 2013, 12: 808-814.
Ba Y, Liu Y, Li P, et al. Spatially resolved electric-field manipulation of magnetism for CoFeB mesoscopic discs on ferroelectrics. Adv Funct Mater 2018, 28: 1706448.
Yu XZ, Onose Y, Kanazawa N, et al. Real-space observation of a two-dimensional skyrmion crystal. Nature 2010, 465: 901-904.
Meguro S, Akahane K, Saito S. Centimeter-order view for magnetic domain imaging with local magnetization direction by longitudinal Kerr effect. AIP Adv 2016, 6: 056504.
Von Hofe T, Urs NO, Mozooni B, et al. Dual wavelength magneto-optical imaging of magnetic thin films. Appl Phys Lett 2013, 103: 142410.
Soldatov IV, Schäfer R. Advances in quantitative Kerr microscopy. Phys Rev B 2017, 95: 014426.
Evans RFL, Hinzke D, Atxitia U, et al. Stochastic form of the Landau-Lifshitz-Bloch equation. Phys Rev B: Condens Matter Mater Phys 2012, 85: 014433.
Hu JM, Nan CW. Electric-field-induced magnetic easy-axis reorientation in ferromagnetic/ferroelectric layered heterostructures. Phys Rev B: Condens Matter Mater Phys 2009, 80: 224416.
Hu JM, Chen LQ, Nan CW. Multiferroic heterostructures integrating ferroelectric and magnetic materials. Adv Mater 2016, 28: 15-39.
Peng RC, Hu JM, Chen LQ, et al. On the speed of piezostrain-mediated voltage-driven perpendicular magnetization reversal: A computational elastodynamics-micromagnetic phase-field study. NPG Asia Mater 2017, 9: e404.
Lo Conte R, Xiao Z, Chen C, et al. Influence of nonuniform micron-scale strain distributions on the electrical reorientation of magnetic microstructures in a composite multiferroic heterostructure. Nano Lett 2018, 18: 1952-1961.
Buzzi M, Chopdekar RV, Hockel JL, et al. Single domain spin manipulation by electric fields in strain coupled artificial multiferroic nanostructures. Phys Rev Lett 2013, 111: 027204
Zhukov A, Ipatov M, Churyukanova M, et al. Giant magnetoimpedance in thin amorphous wires: From manipulation of magnetic field dependence to industrial applications. J Alloys Compd 2014, 586: S279-S286.
Lage E, Kirchhof C, Hrkac V, et al. Exchange biasing of magnetoelectric composites. Nat Mater 2012, 11: 523-529.
Journal of Advanced Ceramics
Pages 1273-1281
Cite this article:
ZHAO X, HU Z, WU J, et al. Vector analysis of electric-field-induced antiparallel magnetic domain evolution in ferromagnetic/ferroelectric heterostructures. Journal of Advanced Ceramics, 2021, 10(6): 1273-1281.








Web of Science






Received: 25 February 2021
Revised: 23 April 2021
Accepted: 17 May 2021
Published: 29 August 2021
© The Author(s) 2021.

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