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Research Article

Efficient synthesis of IrPtPdNi/GO nanocatalysts for superior performance in water electrolysis

Sanha Jang1,§Young Hwa Yun2,§Jin Gyu Lee1Kyung Hee Oh1Shin Wook Kang1Jung-Il Yang1MinJoong Kim2,3Changsoo Lee2,3( )Ji Chan Park1,3( )
Clean Fuel Research Laboratory, Korea Institute of Energy Research, Daejeon 34129, Republic of Korea
Hydrogen Research Department, Korea Institute of Energy Research, Daejeon 34129, Republic of Korea
Energy Engineering, University of Science and Technology, Daejeon 34113, Republic of Korea

§ Sanha Jang and Young Hwa Yun contributed equally to this work.

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Abstract

Traditional iridium (Ir) oxide catalysts have faced significant limitations in water electrolysis, particularly under acidic conditions where instability and degradation severely restrict the efficiency of the oxygen evolution reaction (OER) and hydrogen evolution reaction (HER). To overcome these challenges, this study successfully synthesized highly dispersed IrPtPdNi alloy nanoparticles on a graphene oxide support using a vertically moving reactor, demonstrating exceptional performance in water electrolysis. These nanoparticles, synthesized via a fast-moving bed pyrolysis method, combine iridium, platinum, palladium, and nickel. They exhibit lower overpotentials in OER and comparable performance in HER to commercial catalysts, while also offering enhanced stability. These results surpass the limitations of traditional catalysts, marking significant progress toward more efficient and sustainable hydrogen production technologies. This advancement is expected to contribute significantly to the development of sustainable energy systems by innovatively enhancing the performance of catalysts in the electrochemical water-splitting process.

Graphical Abstract

A rapid synthesis method with a moving reactor was used to develop IrPtPdNi/graphene oxide (GO) nanocatalysts, which showed superior performance in oxygen evolution reaction (OER) and hydrogen evolution reaction (HER), offering new prospects in electrochemistry.

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Nano Research
Pages 10208-10215

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Cite this article:
Jang S, Yun YH, Lee JG, et al. Efficient synthesis of IrPtPdNi/GO nanocatalysts for superior performance in water electrolysis. Nano Research, 2024, 17(11): 10208-10215. https://doi.org/10.1007/s12274-024-6900-6
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Received: 20 May 2024
Revised: 10 July 2024
Accepted: 18 July 2024
Published: 08 August 2024
© Tsinghua University Press 2024