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Research Article

Unveiling strain-enhanced moiré exciton localization in twisted van der Waals homostructures

Henry Rui He1,§Haihong Zheng1,2,§Biao Wu1Shaofei Li1Junnan Ding1Zongwen Liu3Jian-Tao Wang4Anlian Pan5Yanping Liu1,6,7( )
Institute of Quantum Physics, School of Physics, Central South University, Changsha 410083, China
State Key Laboratory of Precision Manufacturing for Extreme Service Performance, Central South University, Changsha 410083, China
School of Chemical and Biomolecular Engineering, The University of Sydney, NSW 2006, Australia
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China
College of Materials Science and Engineering, Hunan University, Changsha 410082, China
State Key Laboratory of High-Performance Complex Manufacturing, Central South University, Changsha 410083, China
Shenzhen Research Institute of Central South University, Shenzhen 51800, China

§ Henry Rui He and Haihong Zheng contributed equally to this work.

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Graphical Abstract

This work explores the interaction between strain and moiré superlattices in twisted 2L-WSe2/2L-WSe2 homobilayers, revealing highly localized moiré-enhanced emission with sharp lines. The study demonstrates the precise control of moiré potential depths through strain engineering, offering insights into the potential for generating strain-induced moiré exciton single-photon sources, thereby advancing quantum emission applications.

Abstract

Moiré superlattices, arising from the controlled twisting of van der Waals homostructures at specific angles, have emerged as a promising platform for quantum emission applications. Concurrently, the manipulation of strain provides a versatile strategy to finely adjust electronic band structures, enhance exciton luminescence efficiency, and establish a robust foundation for two-dimensional quantum light sources. However, the intricate interplay between strain and moiré potential remains partially unexplored. Here, we introduce a meticulously designed fusion of strain engineering and the twisted 2L-WSe2/2L-WSe2 homobilayers, resulting in the precise localization of moiré excitons. Employing low-temperature photoluminescence spectroscopy, we unveil the emergence of highly localized moiré-enhanced emission, characterized by the presence of multiple distinct emission lines. Furthermore, our investigation demonstrates the effective regulation of moiré potential depths through strain engineering, with the potential depths of strained and unstrained regions differing by 91%. By combining both experimental and theoretical approaches, our study elucidates the complex relationship between strain and moiré potential, thereby opening avenues for generating strain-induced moiré exciton single-photon sources.

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Nano Research
Pages 3245-3252
Cite this article:
He HR, Zheng H, Wu B, et al. Unveiling strain-enhanced moiré exciton localization in twisted van der Waals homostructures. Nano Research, 2024, 17(4): 3245-3252. https://doi.org/10.1007/s12274-023-6205-x
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Received: 24 August 2023
Revised: 14 September 2023
Accepted: 14 September 2023
Published: 24 October 2023
© Tsinghua University Press 2023
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