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Nano Research 2024, 17(3): 913-926 https://doi.org/10.1007/s12274-023-6168-y
Research Article | Issue | Published: 27 October 2023

Design of novel RGO/2D strip-like ZIF-8/DMAOP ternary hybrid structure towards high-efficiency microwave absorption, active and passive anti-corrosion, and synergistic antibacterial performance

Show Author's Information Tanlin Chen1,  Yingrui Tian1,  Zihao Guo1,  Yao Chen1,  Qing Qi1( ),  Fanbin Meng1,2( )
Key Laboratory of Advanced Technologies of Materials (Ministry of Education), School of Materials Science and Engineering, Southwest Jiaotong University, Chengdu 610031, China
Shenzhen Institute of Southwest Jiaotong University, Shenzhen 518000, China
Keywords:
microwave absorption, antibacterial, active and passive anti-corrosion, two-dimensional (2D) strip-like zeolitic imidazolate framework-8 (ZIF-8)
Topics:
Graphene
Cite this article:
Chen T, Tian Y, Guo Z, et al. Design of novel RGO/2D strip-like ZIF-8/DMAOP ternary hybrid structure towards high-efficiency microwave absorption, active and passive anti-corrosion, and synergistic antibacterial performance. Nano Research, 2024, 17(3): 913-926. https://doi.org/10.1007/s12274-023-6168-y
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Abstract Full text Electronic supplementary material About this article

In order to meet the requirements of the marine environment for microwave absorption (MA) materials, we put forward the strategy of constructing multi-functional composite materials, which integrate microwave absorption, anti-corrosion, and antibacterial properties. Herein, graphene oxide (GO) was used as a template to induce the growth of zeolitic imidazolate framework-8 (ZIF-8), simultaneously as a two-dimensional (2D) nanocontainers to load corrosion inhibitors to achieve pH-responsive and self-healing properties. Finally, quaternary ammonium salt (dimethyl octadecyl(3-trimethoxylsilyl propyl) ammonium chloride (DMAOP)) and sodium ascorbate (VCNa) were introduced to achieve synergistic antibacterial activity and the reduction of GO. The 2D strip-like structure of ZIF-8 was due to the confined growth induced by the electrostatic attraction between ZIF-8 and GO sheets. The as-obtained reduced GO (RGO)/ZIF-8/DMAOP5 exhibited excellent microwave absorption (MA) properties, with a minimum reflection loss (RL) value of −47.08 dB at 12.73 GHz when the thickness was 2.8 mm. Moreover, the effective absorption bandwidth reached 6.84 GHz. After soaking in 3.5% NaCl solution for 35 days, the RGO/ZIF-8/DMAOP5-0.7% coating still achieved an impedance value of 4.585 × 107 Ω·cm2 and a protective efficiency of 99.994%, providing superior anti-corrosion properties. In addition, fantastic antibacterial activity was obtained, with the antibacterial rates of RGO/ZIF-8/DMAOP10 reaching 99.39% and 100% against Escherichia coli and Staphylococcus aureus. This work could open new avenues towards the development of a new generation of multifunctional MA materials.


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Abstract
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Electronic supplementary material
About this article

Design of novel RGO/2D strip-like ZIF-8/DMAOP ternary hybrid structure towards high-efficiency microwave absorption, active and passive anti-corrosion, and synergistic antibacterial performance

Show Author's information Tanlin Chen1, Yingrui Tian1, Zihao Guo1, Yao Chen1, Qing Qi1( ), Fanbin Meng1,2( )
Key Laboratory of Advanced Technologies of Materials (Ministry of Education), School of Materials Science and Engineering, Southwest Jiaotong University, Chengdu 610031, China
Shenzhen Institute of Southwest Jiaotong University, Shenzhen 518000, China

Abstract

In order to meet the requirements of the marine environment for microwave absorption (MA) materials, we put forward the strategy of constructing multi-functional composite materials, which integrate microwave absorption, anti-corrosion, and antibacterial properties. Herein, graphene oxide (GO) was used as a template to induce the growth of zeolitic imidazolate framework-8 (ZIF-8), simultaneously as a two-dimensional (2D) nanocontainers to load corrosion inhibitors to achieve pH-responsive and self-healing properties. Finally, quaternary ammonium salt (dimethyl octadecyl(3-trimethoxylsilyl propyl) ammonium chloride (DMAOP)) and sodium ascorbate (VCNa) were introduced to achieve synergistic antibacterial activity and the reduction of GO. The 2D strip-like structure of ZIF-8 was due to the confined growth induced by the electrostatic attraction between ZIF-8 and GO sheets. The as-obtained reduced GO (RGO)/ZIF-8/DMAOP5 exhibited excellent microwave absorption (MA) properties, with a minimum reflection loss (RL) value of −47.08 dB at 12.73 GHz when the thickness was 2.8 mm. Moreover, the effective absorption bandwidth reached 6.84 GHz. After soaking in 3.5% NaCl solution for 35 days, the RGO/ZIF-8/DMAOP5-0.7% coating still achieved an impedance value of 4.585 × 107 Ω·cm2 and a protective efficiency of 99.994%, providing superior anti-corrosion properties. In addition, fantastic antibacterial activity was obtained, with the antibacterial rates of RGO/ZIF-8/DMAOP10 reaching 99.39% and 100% against Escherichia coli and Staphylococcus aureus. This work could open new avenues towards the development of a new generation of multifunctional MA materials.

Keywords: microwave absorption, antibacterial, active and passive anti-corrosion, two-dimensional (2D) strip-like zeolitic imidazolate framework-8 (ZIF-8)

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Publication history
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Acknowledgements

Publication history

Received: 22 August 2023
Revised: 04 September 2023
Accepted: 04 September 2023
Published: 27 October 2023
Issue date: March 2024

Copyright

© Tsinghua University Press 2023

Acknowledgements

Acknowledgements

This work was financially supported by the National Natural Science Foundation of China (Nos. 51903213 and 5217130190), the Science and Technology Planning Project of Sichuan Province (Nos. 2023NSFSC1952 and 2022ZYD0028), the Central Government Guides Local Science and Technology Development Special Funds to freely explore basic research projects (No. 2021Szvup124), and the Fundamental Research Funds for the Central Universities (No. 2682021GF004). The authors would like to thank the Analytical and Testing Center of Southwest Jiaotong University for supporting the relative measurements.

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