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Nano Research 2024, 17(3): 1585-1594 https://doi.org/10.1007/s12274-023-6044-9
Research Article | Issue | Published: 30 August 2023

Direct ink writing of multifunctional gratings with gel-like MXene/norepinephrine ink for dynamic electromagnetic interference shielding and patterned Joule heating

Show Author's Information Pei-Zhu Jiang1,2,  Zhiming Deng1,  Peng Min2( ),  Lvxuan Ye1,  Cheng-Zhang Qi1,  Hao-Yu Zhao2,  Ji Liu3,  Hao-Bin Zhang1( ),  Zhong-Zhen Yu2( )
Beijing Key Laboratory of Advanced Functional Polymer Composites, Beijing University of Chemical Technology, Beijing 100029, China
State Key Laboratory of Organic-Inorganic Composites, College of Materials Science and Engineering, Beijing University of Chemical Technology, Beijing 100029, China
School of Chemistry, CRANN and AMBER, Trinity College Dublin, Dublin D02PN40, Ireland
Keywords:
electromagnetic interference shielding, Joule heating, direct ink writing, MXene ink, multifunctional gratings
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Jiang P-Z, Deng Z, Min P, et al. Direct ink writing of multifunctional gratings with gel-like MXene/norepinephrine ink for dynamic electromagnetic interference shielding and patterned Joule heating. Nano Research, 2024, 17(3): 1585-1594. https://doi.org/10.1007/s12274-023-6044-9
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Abstract Full text Electronic supplementary material About this article

Intelligent electromagnetic interference (EMI) shielding modulators with a wide tuning range and cyclic stability are urgently needed but their fabrication remains challenging. A gel-like MXene/norepinephrine ink is developed and multifunctional MXene gratings with wide EMI shielding effectiveness (SE) tuning range, superior reversibility, and high mechanical flexibility are constructed by direct ink writing approach for dynamic EMI shielding and patterned Joule heating applications. The modulable MXene/norepinephrine grating with a high conductivity of 3510 S·cm−1 can conveniently realize the seamless modulation of the EMI SE by adjusting the angle between the MXene grating filaments and the electric field of the incident electromagnetic waves, offering highly reversible switching between shielding “On” (28.0 dB) and “Off” (0.5 dB) states. Notably, due to the optimized integration of the MXene ink and the rationally designed pattern, a superior specific EMI SE of 95,688.2 dB·cm2·g−1 is achieved in the “On” state. Furthermore, the MXene/norepinephrine ink can be used to fabricate many complex patterned gratings with superior stability, instant responsibility, and superb mechanical flexibility, exhibiting a unique patterned Joule heating behavior. Direct writing of multifunctional gratings paves a means for developing intelligent EMI shielding materials, wearable electronic devices, and advanced thermal management materials.


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Electronic supplementary material
About this article

Direct ink writing of multifunctional gratings with gel-like MXene/norepinephrine ink for dynamic electromagnetic interference shielding and patterned Joule heating

Show Author's information Pei-Zhu Jiang1,2, Zhiming Deng1, Peng Min2( ), Lvxuan Ye1, Cheng-Zhang Qi1, Hao-Yu Zhao2, Ji Liu3, Hao-Bin Zhang1( ), Zhong-Zhen Yu2( )
Beijing Key Laboratory of Advanced Functional Polymer Composites, Beijing University of Chemical Technology, Beijing 100029, China
State Key Laboratory of Organic-Inorganic Composites, College of Materials Science and Engineering, Beijing University of Chemical Technology, Beijing 100029, China
School of Chemistry, CRANN and AMBER, Trinity College Dublin, Dublin D02PN40, Ireland

Abstract

Intelligent electromagnetic interference (EMI) shielding modulators with a wide tuning range and cyclic stability are urgently needed but their fabrication remains challenging. A gel-like MXene/norepinephrine ink is developed and multifunctional MXene gratings with wide EMI shielding effectiveness (SE) tuning range, superior reversibility, and high mechanical flexibility are constructed by direct ink writing approach for dynamic EMI shielding and patterned Joule heating applications. The modulable MXene/norepinephrine grating with a high conductivity of 3510 S·cm−1 can conveniently realize the seamless modulation of the EMI SE by adjusting the angle between the MXene grating filaments and the electric field of the incident electromagnetic waves, offering highly reversible switching between shielding “On” (28.0 dB) and “Off” (0.5 dB) states. Notably, due to the optimized integration of the MXene ink and the rationally designed pattern, a superior specific EMI SE of 95,688.2 dB·cm2·g−1 is achieved in the “On” state. Furthermore, the MXene/norepinephrine ink can be used to fabricate many complex patterned gratings with superior stability, instant responsibility, and superb mechanical flexibility, exhibiting a unique patterned Joule heating behavior. Direct writing of multifunctional gratings paves a means for developing intelligent EMI shielding materials, wearable electronic devices, and advanced thermal management materials.

Keywords: electromagnetic interference shielding, Joule heating, direct ink writing, MXene ink, multifunctional gratings

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Publication history
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Acknowledgements

Publication history

Received: 04 July 2023
Revised: 21 July 2023
Accepted: 26 July 2023
Published: 30 August 2023
Issue date: March 2024

Copyright

© Tsinghua University Press 2023

Acknowledgements

Acknowledgements

The financial support from the National Natural Science Foundation of China (Nos. 51922020, 52090034 and 52221006), and the Open Fund of State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology (No. OIC-202201001) is gratefully acknowledged.

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