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Research Article

Diameter-dependent photoelectric performances of semiconducting carbon nanotubes/perovskite heterojunctions

Yayang Yu1,2, Wenke Wang2,3,4, Xiao Li2,3,4, Linhai Li2,3,4, Shilong Li2,4, Xiaojun Wei2,3,4,5, Weiya Zhou2,3,4,5, Jing Lin1, Yang Huang1( ), Huaping Liu2,3,4,5( )
School of Materials Science and Engineering, Hebei Key Laboratory of Boron Nitride Micro and Nano Materials, Hebei University of Technology, Tianjin 300130, China
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China
Center of Materials Science and Optoelectronics Engineering, School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 100049, China
Beijing Key Laboratory for Advanced Functional Materials and Structure Research, Beijing 100190, China
Songshan Lake Materials Laboratory, Dongguan 523808, China
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Graphical Abstract

The responsivity, detectivity, and response speed of single-wall carbon nanotubes (SWCNTs)/CsPbBr3 quantum dots (QDs) heterojunction photodetectors increase with an increase in SWCNT diameter.

Abstract

The heterojunction of single-wall carbon nanotubes (SWCNTs) and perovskite quantum dots (QDs) shows excellent photodetection performances due to the combination of the advantages of high carrier mobility of SWCNTs and high absorption coefficient of perovskite QDs. However, the band structure of a SWCNT is determined by its atomic arrangement structure. How the structure of SWCNTs affects the photoelectric performance of the composite film remains elusive. Here, we systematically explored the diameter effect of SWCNTs with different bandgaps on the photodetection performances of SWCNTs/perovskite QDs heterojunction films by integrating semiconducting SWCNTs (s-SWCNTs) with different diameters with CsPbBr3 QDs. The results show that with an increase in diameter of s-SWCNTs, the heterojunction exhibits increasing responsivity (R), detectivity (D*), and faster response time. The great improvement in the optoelectronic performances of devices should be attributed to the higher carrier mobility of larger-diameter SWCNT films and the increasing built-in electric field at the heterojunction interfaces between larger-diameter SWCNTs and CsPbBr3 QDs, which enhances the separation of the photogenerated excitons and the transport of the resulted carriers in SWCNT films.

Keywords

carbon nanotubesperovskite quantum dotsdiameter effectresponsivitydetectivity

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Nano Research
Volume 16 Issue 11,
November 2023
Pages 12662-12669
DOI: 10.1007/s12274-023-5942-1
Cite this article:
Yu Y, Wang W, Li X, et al. Diameter-dependent photoelectric performances of semiconducting carbon nanotubes/perovskite heterojunctions. Nano Research, 2023, 16(11): 12662-12669. https://doi.org/10.1007/s12274-023-5942-1
Topics:
Carbon nanotubesPhotodetectorsSemiconductor quantum dots

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Received: 01 May 2023
Revised: 17 June 2023
Accepted: 20 June 2023
Published: 27 July 2023
© Tsinghua University Press 2023
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