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Nano Research 2023, 16(2): 3451-3474 https://doi.org/10.1007/s12274-022-4859-4
Review Article | Issue | Published: 02 September 2022

Recent advances on the construction of encapsulated catalyst for catalytic applications

Show Author's Information Minghui Li1,2,  Yaning Yang1,  Dailiang Yu1,  Wenwen Li1,  Xin Ning3,  Rui Wan1,  Hongjie Zhu4,  Junjie Mao2( )
School of Ecology and Environment, Anhui Normal University, Wuhu 241002, China
Key Laboratory of Functional Molecular Solids, Ministry of Education, College of Chemistry and Materials Science, Anhui Normal University, Wuhu 241002, China
College of Environmental Science and Engineering, Yangzhou University, Yangzhou 225127, China
Shandong Provincial Key Laboratory of Chemical Energy Storage and Novel Cell Technology, School of Chemistry and Chemical Engineering, Liaocheng University, Liaocheng 252059, China
Keywords:
heterogeneous catalysis, catalyst design, catalytic performance, encapsulated catalyst, deactivation
Topics:
Synthesis
Cite this article:
Li M, Yang Y, Yu D, et al. Recent advances on the construction of encapsulated catalyst for catalytic applications. Nano Research, 2023, 16(2): 3451-3474. https://doi.org/10.1007/s12274-022-4859-4
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Abstract Full text Electronic supplementary material About this article

In heterogeneous catalytic reactions, supported metal catalysts have attracted increasing attention for the environmental remediation and industrial manufacture due to their inherent catalytic capacity. However, leaching, agglomeration, and poisoning of active metal particles lead to catalyst deactivation, thereby limiting their applications. To avoid this, strategies to protect the active metals from such inactivating processes are major areas of research. Emerging encapsulation strategies, in which active species are coated by protective shells, have proven to be a powerful technology to enhance catalytic performance by creating a well-developed structure about the active catalytic sites. This review highlights the recent advances on preparation method and application of encapsulated catalysts since 2016. Building upon the traditional confinement effect, new categories and extended concepts of encapsulation are introduced. In parallel, effects of encapsulation structure on performance and key factors controlling the structure of encapsulated catalyst are discussed definitely in this review. Finally, future perspectives on opportunities and challenges for further research in the field are given at the end of this paper.


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Abstract
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Electronic supplementary material
About this article

Recent advances on the construction of encapsulated catalyst for catalytic applications

Show Author's information Minghui Li1,2, Yaning Yang1, Dailiang Yu1, Wenwen Li1, Xin Ning3, Rui Wan1, Hongjie Zhu4, Junjie Mao2( )
School of Ecology and Environment, Anhui Normal University, Wuhu 241002, China
Key Laboratory of Functional Molecular Solids, Ministry of Education, College of Chemistry and Materials Science, Anhui Normal University, Wuhu 241002, China
College of Environmental Science and Engineering, Yangzhou University, Yangzhou 225127, China
Shandong Provincial Key Laboratory of Chemical Energy Storage and Novel Cell Technology, School of Chemistry and Chemical Engineering, Liaocheng University, Liaocheng 252059, China

Abstract

In heterogeneous catalytic reactions, supported metal catalysts have attracted increasing attention for the environmental remediation and industrial manufacture due to their inherent catalytic capacity. However, leaching, agglomeration, and poisoning of active metal particles lead to catalyst deactivation, thereby limiting their applications. To avoid this, strategies to protect the active metals from such inactivating processes are major areas of research. Emerging encapsulation strategies, in which active species are coated by protective shells, have proven to be a powerful technology to enhance catalytic performance by creating a well-developed structure about the active catalytic sites. This review highlights the recent advances on preparation method and application of encapsulated catalysts since 2016. Building upon the traditional confinement effect, new categories and extended concepts of encapsulation are introduced. In parallel, effects of encapsulation structure on performance and key factors controlling the structure of encapsulated catalyst are discussed definitely in this review. Finally, future perspectives on opportunities and challenges for further research in the field are given at the end of this paper.

Keywords: heterogeneous catalysis, catalyst design, catalytic performance, encapsulated catalyst, deactivation

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Publication history
Copyright
Acknowledgements

Publication history

Received: 08 July 2022
Revised: 29 July 2022
Accepted: 02 August 2022
Published: 02 September 2022
Issue date: February 2023

Copyright

© Tsinghua University Press 2022

Acknowledgements

Acknowledgements

This work was supported by the National Natural Science Foundation of China (Nos. 21971002 and 42077361), the Natural Science Foundation of Anhui Province (No. 1908085QB45), Open Fund of State Key Lab of Pollution Control and Resource Reuse Research, China (No. PCRRF20002), and the University Natural Science Research Project of Anhui Province (No. KJ2020A0064).

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