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Nano Research 2022, 15(10): 9520-9530 https://doi.org/10.1007/s12274-022-4756-x
Research Article | Issue | Published: 05 August 2022

Robust double-layered ANF/MXene-PEDOT:PSS Janus films with excellent multi-source driven heating and electromagnetic interference shielding properties

Show Author's Information Bing Zhou,  Jianzhou Song,  Bo Wang,  Yuezhan Feng( ),  Chuntai Liu( ),  Changyu Shen
Key Laboratory of Materials Processing and Mold Ministry of Education, National Engineering Research Center for Advanced Polymer Processing Technology, Zhengzhou University, Zhengzhou 450002, China
Keywords:
mechanical properties, MXene, double-layer structure, electromagnetic interference (EMI) shielding, electro-/photothermal conversion
Topics:
Conductive films
Cite this article:
Zhou B, Song J, Wang B, et al. Robust double-layered ANF/MXene-PEDOT:PSS Janus films with excellent multi-source driven heating and electromagnetic interference shielding properties. Nano Research, 2022, 15(10): 9520-9530. https://doi.org/10.1007/s12274-022-4756-x
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Abstract Full text Electronic supplementary material About this article

The strategy of incorporating polymers into MXene-based functional materials has been widely used to improve their mechanical properties, however with inevitable sacrifice of their electrical conductivity and electromagnetic interference (EMI) shielding performance. This study demonstrates a facile yet efficient layering structure design to prepare the highly robust and conductive double-layer Janus films comprised of independent aramid nanofiber (ANF) and Ti3C2Tx MXene/poly(3,4-ethylenedioxy- thiophene):poly(styrenesulfonate) (PEDOT:PSS) layers. The ANF layer serves to provide good mechanical stability, whilst the MXene/PEDOT:PSS layer ensures excellent electrical conductivity. Doping PEDOT:PSS into the MXene layer enhances the interfacial bonding strength between the MXene and ANF layers and improves the hydrophobicity and water/oxidation resistance of MXene layer. The resultant ANF/MXene-PEDOT:PSS Janus film with a conductive layer thickness of 4.4 μm was shown to display low sheet resistance (2.18 Ω/sq), good EMI shielding effectiveness (EMI SE of 48.1 dB), high mechanical strength (155.9 MPa), and overall toughness (19.4 MJ/m3). Moreover, the excellent electrical conductivity and light absorption capacity of the MXene-PEDOT:PSS conductive layer mean that these Janus films display multi-source driven heating functions, producing excellent Joule heating (382 °C at 4 V) and photothermal conversion (59.6 °C at 100 mW/m2) properties.


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About this article

Robust double-layered ANF/MXene-PEDOT:PSS Janus films with excellent multi-source driven heating and electromagnetic interference shielding properties

Show Author's information Bing Zhou, Jianzhou Song, Bo Wang, Yuezhan Feng( ), Chuntai Liu( ), Changyu Shen
Key Laboratory of Materials Processing and Mold Ministry of Education, National Engineering Research Center for Advanced Polymer Processing Technology, Zhengzhou University, Zhengzhou 450002, China

Abstract

The strategy of incorporating polymers into MXene-based functional materials has been widely used to improve their mechanical properties, however with inevitable sacrifice of their electrical conductivity and electromagnetic interference (EMI) shielding performance. This study demonstrates a facile yet efficient layering structure design to prepare the highly robust and conductive double-layer Janus films comprised of independent aramid nanofiber (ANF) and Ti3C2Tx MXene/poly(3,4-ethylenedioxy- thiophene):poly(styrenesulfonate) (PEDOT:PSS) layers. The ANF layer serves to provide good mechanical stability, whilst the MXene/PEDOT:PSS layer ensures excellent electrical conductivity. Doping PEDOT:PSS into the MXene layer enhances the interfacial bonding strength between the MXene and ANF layers and improves the hydrophobicity and water/oxidation resistance of MXene layer. The resultant ANF/MXene-PEDOT:PSS Janus film with a conductive layer thickness of 4.4 μm was shown to display low sheet resistance (2.18 Ω/sq), good EMI shielding effectiveness (EMI SE of 48.1 dB), high mechanical strength (155.9 MPa), and overall toughness (19.4 MJ/m3). Moreover, the excellent electrical conductivity and light absorption capacity of the MXene-PEDOT:PSS conductive layer mean that these Janus films display multi-source driven heating functions, producing excellent Joule heating (382 °C at 4 V) and photothermal conversion (59.6 °C at 100 mW/m2) properties.

Keywords: mechanical properties, MXene, double-layer structure, electromagnetic interference (EMI) shielding, electro-/photothermal conversion

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Publication history
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Publication history

Received: 10 June 2022
Revised: 01 July 2022
Accepted: 10 July 2022
Published: 05 August 2022
Issue date: October 2022

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