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Nano Research 2022, 15(7): 6128-6137 https://doi.org/10.1007/s12274-022-4198-5
Research Article | Issue | Published: 29 March 2022

Tunable ultrathin dual-phase P-doped Bi2MoO6 nanosheets for advanced lithium and sodium storage

Show Author's Information Fucong Lyu1,2,5,6,  Zhe Jia3,5,  Shanshan Zeng7,8,  Fei-Xiang Ma1,5,  Lulu Pan1,5,  Lizi Cheng1,5,  Yan Bao1,5,  Ligang Sun4,5,  Weihui Ou2,5,7,  Peng Du7,8,  Yang Yang Li7,8( ),  Jian Lu1,2,5,6 ( )
Centre for Advanced Structural Materials, City University of Hong Kong Shenzhen Research Institute, Greater Bay Joint Division, Shenyang National Laboratory for Materials Science, Shenzhen 518057, China
Hong Kong Branch of National Precious Metals Material Engineering Research Centre, City University of Hong Kong, Kowloon, Hong Kong, China
School of Materials Science and Engineering, Southeast University, Nanjing 211189, China
School of Science, Harbin Institute of Technology, Shenzhen 518055, China
Department of Mechanical Engineering, City University of Hong Kong, Kowloon, Hong Kong, China
CityU-Shenzhen Futian Research Institute, Shenzhen 518045, China
Center of Super-Diamond and Advanced Films (COSDAF), City University of Hong Kong, Kowloon, Hong Kong, China
Department of Material Science and Engineering, City University of Hong Kong, Kowloon, Hong Kong, China
Keywords:
sodium-ion batteries, lithium-ion batteries, ultrathin nanosheets, anode materials, amorphous/nanocrystalline dual-phase structure, P-doped Bi2MoO6
Topics:
Energy
Cite this article:
Lyu F, Jia Z, Zeng S, et al. Tunable ultrathin dual-phase P-doped Bi2MoO6 nanosheets for advanced lithium and sodium storage. Nano Research, 2022, 15(7): 6128-6137. https://doi.org/10.1007/s12274-022-4198-5
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Abstract Full text Electronic supplementary material About this article

The construction of electrode materials for lithium-ion batteries (LIBs) and sodium-ion batteries (SIBs) has gradually been an appealing and attractive technology in energy storage research field. In the present work, a facile strategy of synthesizing ultrathin amorphous/nanocrystal dual-phase P-doped Bi2MoO6 (denoted as P-BiMO) nanosheets via a one-step wet-chemical synthesis approach is explored. Quite distinct from conventional two-dimensional (2D) nanosheets, our newly developed ultrathin P-BiMO nanosheets exhibit a unique tunable amorphous/nanocrystalline dual-phase structure with several compelling advantages including fast ion exchange ability and superb volume change buffer capability. The experimental results reveal that our prepared P-BiMO-6 electrode delivers an excellent reversible capacity of 509.6 mA·g−1 after continuous 1,500 cycles at the current densities of 1,500 mA·g−1 and improved rate performance for LIBs. In the meanwhile, the P-BiMO-6 electrode also shows a reversible capacity of 300.6 mA·g−1 after 100 cycles at 50 mA·g−1 when being used as the SIBs electrodes. This present work uncovers an effective dual-phase nanosheet structure to improve the performance of batteries, providing an attractive paradigm to develop superior electrode materials.


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Electronic supplementary material
About this article

Tunable ultrathin dual-phase P-doped Bi2MoO6 nanosheets for advanced lithium and sodium storage

Show Author's information Fucong Lyu1,2,5,6, Zhe Jia3,5, Shanshan Zeng7,8, Fei-Xiang Ma1,5, Lulu Pan1,5, Lizi Cheng1,5, Yan Bao1,5, Ligang Sun4,5, Weihui Ou2,5,7, Peng Du7,8, Yang Yang Li7,8( ), Jian Lu1,2,5,6 ( )
Centre for Advanced Structural Materials, City University of Hong Kong Shenzhen Research Institute, Greater Bay Joint Division, Shenyang National Laboratory for Materials Science, Shenzhen 518057, China
Hong Kong Branch of National Precious Metals Material Engineering Research Centre, City University of Hong Kong, Kowloon, Hong Kong, China
School of Materials Science and Engineering, Southeast University, Nanjing 211189, China
School of Science, Harbin Institute of Technology, Shenzhen 518055, China
Department of Mechanical Engineering, City University of Hong Kong, Kowloon, Hong Kong, China
CityU-Shenzhen Futian Research Institute, Shenzhen 518045, China
Center of Super-Diamond and Advanced Films (COSDAF), City University of Hong Kong, Kowloon, Hong Kong, China
Department of Material Science and Engineering, City University of Hong Kong, Kowloon, Hong Kong, China

Abstract

The construction of electrode materials for lithium-ion batteries (LIBs) and sodium-ion batteries (SIBs) has gradually been an appealing and attractive technology in energy storage research field. In the present work, a facile strategy of synthesizing ultrathin amorphous/nanocrystal dual-phase P-doped Bi2MoO6 (denoted as P-BiMO) nanosheets via a one-step wet-chemical synthesis approach is explored. Quite distinct from conventional two-dimensional (2D) nanosheets, our newly developed ultrathin P-BiMO nanosheets exhibit a unique tunable amorphous/nanocrystalline dual-phase structure with several compelling advantages including fast ion exchange ability and superb volume change buffer capability. The experimental results reveal that our prepared P-BiMO-6 electrode delivers an excellent reversible capacity of 509.6 mA·g−1 after continuous 1,500 cycles at the current densities of 1,500 mA·g−1 and improved rate performance for LIBs. In the meanwhile, the P-BiMO-6 electrode also shows a reversible capacity of 300.6 mA·g−1 after 100 cycles at 50 mA·g−1 when being used as the SIBs electrodes. This present work uncovers an effective dual-phase nanosheet structure to improve the performance of batteries, providing an attractive paradigm to develop superior electrode materials.

Keywords: sodium-ion batteries, lithium-ion batteries, ultrathin nanosheets, anode materials, amorphous/nanocrystalline dual-phase structure, P-doped Bi2MoO6

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Publication history
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Acknowledgements

Publication history

Received: 13 December 2021
Revised: 17 January 2022
Accepted: 20 January 2022
Published: 29 March 2022
Issue date: July 2022

Copyright

© Tsinghua University Press 2022

Acknowledgements

Acknowledgements

This work is supported by Shenzhen-Hong Kong Science and Technology Innovation Cooperation Zone Shenzhen Park Project: HZQB-KCZYB-2020030, the National Key R&D Program of China (Project No. 2017YFA0204403), Hong Kong Innovation and Technology Commission via the Hong Kong Branch of National Precious Metals Material Engineering Research Center.

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