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It is of great importance to develop facile strategies to synthesize catalysts with desirable compositions and structures for high-performance photocatalytic hydrogen generation. In this work, we put forward an ionic liquid assisted one-pot route for the synthesis of heteroatom-doped Pt/TiO2 composite material. This route is simple, environmentally benign and adjustable owing to the designable properties of ionic liquids. The as-synthesized Pt/TiO2 nanocrystals exhibit high activity and stability for the photocatalytic hydrogen generation under simulated solar irradiation. This method can be easily applied to the synthesis of various kinds of metal/TiO2 composites doped with desirable heteroatoms (e.g., F, Cl, Br, etc).

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Publication history
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Acknowledgements

Publication history

Received: 28 March 2019
Revised: 06 June 2019
Accepted: 27 June 2019
Published: 10 July 2019
Issue date: August 2019

Copyright

© Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2019

Acknowledgements

Acknowledgements

The authors thank the financial supports from the National Natural Science Foundation of China (Nos. 21525316 and 21673254), Ministry of Science and Technology of China (No. 2017YFA0403003), Chinese Academy of Sciences (No. QYZDY-SSW-SLH013), and Beijing Municipal Science & Technology Commission (No. Z181100004218004).

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