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Research Article

Synthesis of Co/SiO2 hybrid nanocatalyst via twisted Co3Si2O5(OH)4 nanosheets for high-temperature Fischer- Tropsch reaction

Ji Chan Park1,2( ), Shin Wook Kang1, Jeong-Chul Kim3, Jae In Kwon1, Sanha Jang1, Geun Bae Rhim1, Mijong Kim4, Dong Hyun Chun1,2, Ho-Tae Lee1, Heon Jung1, Hyunjoon Song4( ), Jung-Il Yang1( )
Clean Fuel LaboratoryKorea Institute of Energy ResearchDaejeon34129Republic of Korea
Advanced Energy TechnologyUniversity of Science and TechnologyDaejeon34113Republic of Korea
Center for Nanomaterials & Chemical ReactionsInstitute for Basic ScienceDaejeon34141Republic of Korea
Department of ChemistryKorea Advanced Institute of Science and TechnologyDaejeon34141Republic of Korea
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Abstract

A cobalt-silica hybrid nanocatalyst bearing small cobalt particles of diameter ~5 nm was prepared through a hydrothermal reaction and hydrogen reduction. The resulting material showed very high CO conversion (> 82%) and high hydrocarbon productivity (~1.0 gHC·gcat-1·h-1) with high activity (~8.5 × 10-5 molCO·gCo-1·s-1) in the Fischer-Tropsch synthesis reaction.

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Keywords

hybrid nanostructureFischer-Tropsch synthesisthermal stabilitymetal silicate hydroxidecobalt catalyst

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Nano Research
Volume 10 Issue 3,
March 2017
Pages 1044-1055
DOI: 10.1007/s12274-016-1364-7

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Park JC, Kang SW, Kim J-C, et al. Synthesis of Co/SiO2 hybrid nanocatalyst via twisted Co3Si2O5(OH)4 nanosheets for high-temperature Fischer- Tropsch reaction. Nano Research, 2017, 10(3): 1044-1055. https://doi.org/10.1007/s12274-016-1364-7

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Received: 29 August 2016
Revised: 23 October 2016
Accepted: 09 November 2016
Published: 11 January 2017
© Tsinghua University Press and Springer-Verlag Berlin Heidelberg 2016