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Research Article

Topological crystalline insulator nanomembrane with strain-tunable band gap

Xiaofeng Qian1Liang Fu2( )Ju Li1 ( )
Department of Nuclear Science and Engineering and Department of Materials Science and EngineeringMassachusetts Institute of TechnologyCambridgeMassachusetts02139USA
Department of PhysicsMassachusetts Institute of TechnologyCambridgeMassachusetts02139USA
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Abstract

The ability to fine-tune band gap and band inversion in topological materials is highly desirable for the development of novel functional devices. Here we propose that the electronic properties of free-standing nanomembranes of the topological crystalline insulators (TCI) SnTe and Pb1-xSnx(Se, Te) are highly tunable by engineering elastic strain and membrane thickness, resulting in tunable band gap and giant piezoconductivity. Membrane thickness governs the hybridization of topological electronic states on opposite surfaces, while elastic strain can further modulate the hybridization strength by controlling the penetration length of surface states. We propose a frequency-resolved infrared photodetector using force-concentration induced inhomogeneous elastic strain in TCI nanomembranes with spatially varying width. The predicted tunable band gap accompanied by strong spin-textured electronic states will open new avenues for fabricating piezoresistive devices, infrared detectors and energy-efficient electronic and spintronic devices based on TCI nanomembrane.

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Nano Research
Pages 967-979

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Cite this article:
Qian X, Fu L, Li J. Topological crystalline insulator nanomembrane with strain-tunable band gap. Nano Research, 2015, 8(3): 967-979. https://doi.org/10.1007/s12274-014-0578-9

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Received: 10 May 2013
Revised: 31 August 2014
Accepted: 06 September 2014
Published: 17 October 2014
© Tsinghua University Press and Springer-Verlag Berlin Heidelberg 2014