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We present a lithography-free technique for fabrication of clean, high quality graphene devices. This technique is based on evaporation through hard Si shadow masks, and eliminates contaminants introduced by lithographical processes. We demonstrate that devices fabricated by this technique have significantly higher mobility values than those obtained by standard electron beam lithography. To obtain ultra-high mobility devices, we extend this technique to fabricate suspended graphene samples with mobilities as high as 120 000 cm2/(V·s).


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Lithography-Free Fabrication of High Quality Substrate-Supported and Freestanding Graphene Devices

Show Author's information Wenzhong Bao1Gang Liu1Zeng Zhao1Hang Zhang1Dong Yan2Aparna Deshpande3Brian LeRoy3Chun Ning Lau1( )
Department of Physics and Astronomy, University of CaliforniaRiverside, CA 92521 USA
Center for Nanoscale Science and Engineering, University of CaliforniaRiverside, CA 92521 USA
Department of Physics, University of ArizonaTucson, AZ 85721 USA

Abstract

We present a lithography-free technique for fabrication of clean, high quality graphene devices. This technique is based on evaporation through hard Si shadow masks, and eliminates contaminants introduced by lithographical processes. We demonstrate that devices fabricated by this technique have significantly higher mobility values than those obtained by standard electron beam lithography. To obtain ultra-high mobility devices, we extend this technique to fabricate suspended graphene samples with mobilities as high as 120 000 cm2/(V·s).

Keywords: mobility, Suspended graphene, shadow mask, lithography-free, e-beam evaporation

References(19)

1

Zhang, Y. B.; Tan, Y. W.; Stormer, H. L.; Kim, P. Experimental observation of the quantum Hall effect and Berry's phase in graphene. Nature 2005, 438, 201–204.

2

Novoselov, K. S.; Geim, A. K.; Morozov, S. V.; Jiang, D.; Katsnelson, M. I.; Grigorieva, I. V.; Dubonos, S. V.; Firsov, A. A. Two-dimensional gas of massless Dirac fermions in graphene. Nature 2005, 438, 197–200.

3

Novoselov, K. S.; Geim, A. K.; Morozov, S. V.; Jiang, D.; Zhang, Y.; Dubonos, S. V.; Grigorieva, I. V.; Firsov, A. A. Electric field effect in atomically thin carbon films. Science 2004, 306, 666–669.

4

Lee, C.; Wei, X. D.; Kysar, J. W.; Hone, J. Measurement of the elastic properties and intrinsic strength of monolayer graphene. Science 2008, 321, 385–388.

5

Bao, W. Z.; Miao, F.; Chen, Z.; Zhang, H.; Jang, W. Y.; Dames, C.; Lau, C. N. Controlled ripple texturing of suspended graphene and ultrathin graphite membranes. Nat. Nanotechnol. 2009, 4, 562–566.

6

Balandin, A. A.; Ghosh, S.; Bao, W. Z.; Calizo, I.; Teweldebrhan, D.; Miao, F.; Lau, C. N. Superior thermal conductivity of single-layer graphene. Nano Lett. 2008, 8, 902–907.

7

Cheianov, V. V.; Fal'ko, V. I. Selective transmission of Dirac electrons and ballistic magnetoresistance of np junctions in graphene. Phys. Rev. B 2006, 74, 041403.

8

Katsnelson, M. I.; Novoselov, K. S.; Geim, A. K. Chiral tunnelling and the Klein paradox in graphene. Nat. Phys. 2006, 2, 620–625.

9

Peres, N. M. R.; Guinea, F.; Neto, A. H. C. Electronic properties of disordered two-dimensional carbon. Phys. Rev. B 2006, 73, 125411.

10

Du, X.; Skachko, I.; Barker, A.; Andrei, E. Y. Approaching ballistic transport in suspended graphene. Nat. Nanotechnol. 2008, 3, 491–495.

11

Bolotin, K. I.; Sikes, K. J.; Jiang, Z.; Fundenberg, G.; Hone, J.; Kim, P.; Stormer, H. L. Ultrahigh electron mobility in suspended graphene. Solid State Comm. 2008, 146, 351–355.

12

Chen, J. H.; Jang, C.; Adam, S.; Fuhrer, M. S.; Williams, E. D.; Ishigami, M. Charged-impurity scattering in graphene. Nat. Phys. 2008, 4, 377–381.

13

Moser, J.; Barreiro, A.; Bachtold, A. Current-induced cleaning of graphene. Appl. Phys. Lett. 2007, 91, 163513.

14

Girit, C. O.; Zettl, A. Soldering to a single atomic layer. Appl. Phys. Lett. 2007, 91, 193512.

15

Staley, N.; Wang, H.; Puls, C.; Forster, J.; Jackson, T. N.; McCarthy, K.; Clouser, B.; Liu, Y. Lithography-free fabrication of graphene devices. Appl. Phys. Lett. 2007, 90, 143518.

16

Deshmukh, M. M.; Ralph, D. C.; Thomas, M.; Silcox, J. Nanofabrication using a stencil mask. Appl. Phys. Lett. 1999, 75, 1631–1633.

17

Zhou Y. X.; Johnson, A. T. Simple fabrication of molecular circuits by shadow mask evaporation. Nano Lett. 2003, 3, 1371–1374.

18

Lishchynska, M.; Bourenkov, V.; van den Boogaart, M. A. F.; Doeswijk, L.; Brugger, J.; Greer, J. C. Predicting mask distortion, clogging and pattern transfer for stencil lithography. Microelectron. Eng. 2007, 84, 42–53.

19

Egger, S.; Ilie, A.; Fu, Y. T.; Chongsathien, J.; Kang, D. J.; Welland, M. E. Dynamic shadow mask technique: A universal tool for nanoscience. Nano Lett. 2005, 5, 15–20.

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Received: 09 November 2009
Revised: 07 December 2009
Accepted: 08 December 2009
Published: 27 March 2010
Issue date: February 2010

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© The Author(s) 2010

Acknowledgements

Acknowledgements

We thank Feng Miao for trench wafer fabrication and Hsinyin Chiu for useful discussion. This work is supported in part by Semiconductor Research Corporation (SRC), Office of Naval Research (ONR) N00014-09-1- 0724, ONR/Defense Microelectronics Activity (DMEA) H94003-09-2-0901, the U. S. Army Research Laboratory and Army Research Office (ARO)/W911NF-09-1-0333.

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