TY - JOUR AU - Kumar, Parveen AU - Nadeem, Irfan AU - Yaqub, Talha Bin AU - Morina, Ardian AU - Kalin, Mitjan PY - 2026 TI - Electrically induced superlubricity of electrophoretically deposited graphene-nanoplatelet coatings under aqueous glycerol-lubricated sliding conditions JO - Friction SN - 2223-7690 AB - Superlubricity has attracted increasing global interest as an effective strategy for reducing friction-related energy losses in response to rising energy demands. This study demonstrates the feasibility of achieving rapid superlubricity on a steel surface coated with graphene nanoplatelets by controlled electrical stimulation under aqueous glycerol lubrication. The results show that a current of +0.1 A promotes the exfoliation and alignment of the graphene nanoplatelets parallel to the sliding direction. This alignment promotes low-shear interlayer sliding, while detached graphene fragments effectively fill the surface asperities and microcracks, enabling continuous mechanical self-healing. As a result, a stable early superlubricity regime was established within 145 s, yielding a coefficient of friction (CoF) of ~0.007, and negligible wear. In contrast, a higher current of 3 A triggers excessive electrochemical oxidation and localised thermal effects that overwhelm the defect-healing capability of graphene, leading to insufficient surface passivation, severe wear, accompanied by 9.28-fold increase in CoF (~0.065). This study introduces a novel lubrication strategy for achieving superlubricity under electrified contact conditions and provides fundamental insights into the practical implementation of graphene-based superlubric systems in electrically driven sliding applications. UR - https://doi.org/10.26599/FRICT.2026.9441335 DO - 10.26599/FRICT.2026.9441335