@article{Liu2026, 
author = {Yulin Liu and Jiaxing Yang and Jie Qu and Hongliu Dai and Chao Lai},
title = {Three-dimensional scaffold-supported hydrogel electrolytes with integrated high conductivity and stability for robust zinc-ion batteries},
year = {2026},
journal = {Nano Research},
volume = {19},
number = {11},
pages = {94909083},
keywords = {zinc-ion battery, hydrogel electrolyte, ionic conductivity, interfacial stability, zinc dendrites},
url = {https://www.sciopen.com/article/10.26599/NR.2026.94909083},
doi = {10.26599/NR.2026.94909083},
abstract = {Hydrogel electrolytes (HGEs) have emerged as promising electrolytes for zinc-ion batteries (ZIBs), owing to their favorable mechanical strength, ionic conductivity, and interfacial stability. However, simultaneously achieving these mutually conflicting properties remains a key issue that hinders their rapid development. Herein, we propose a molecular-scale strategy to precisely balance these mutually conflicting properties in HGEs using sucrose and choline chloride. Our findings reveal that the synergistically modified HGE, achieving a high hydrogen production inhibition rate of 97.2%, high ionic conductivity of 17.71 mS·cm−1, high mechanical properties (strength of 278.07 kPa, elongation of 463.62%), enabling the Zn anode to reach an average Coulombic efficiency (CE) of 99.16% over 700 cycles and maintain highly reversible cycling for up to 1300 h at a high current density of 5 mA·cm−2. This study presents a promising strategy for developing a green, high-performance HGE, which is expected to accelerate the practical implementation of ZIBs.}
}