TY - JOUR AU - Zou, Bo AU - Zhou, Yu AU - Zhou, Yan AU - Wu, Yanyan AU - He, Yang AU - Wang, Xiaonan AU - Yang, Jinfeng AU - Zhang, Lianghui AU - Chen, Yuxiang AU - Zhou, Shi AU - Guo, Huaixin AU - Sun, Huarui PY - 2022 TI - Reliable and broad-range layer identification of Au-assisted exfoliated large area MoS2 and WS2 using reflection spectroscopic fingerprints JO - Nano Research SN - 1998-0124 SP - 8470 EP - 8478 VL - 15 IS - 9 AB - The emerging Au-assisted exfoliation technique enables the production of a wealth of large-area and high-quality ultrathin two dimensional (2D) crystals. Fast, damage-free, and reliable determination of the layer number of such 2D films can greatly promote layer-dependent physical studies and device applications. Here, an optical method has been developed for simple, high throughput, and accurate determination of the layer number for Au-assisted exfoliated MoS2 and WS2 films in a broad thickness range. The method is based on quantitative analysis of layer-dependent white light reflection spectra (WLRS), revealing that the intensity of exciton-induced reflection peaks can be used as a clear indicator for identifying the layer number. The simple yet robust method will facilitate fundamental studies on layer-dependent optical, electrical, and thermal properties and device applications of 2D materials. The technique can also be readily combined with photoluminescence (PL) and Raman spectroscopies to study other layer-dependent physical properties of 2D materials. UR - https://doi.org/10.1007/s12274-022-4418-z DO - 10.1007/s12274-022-4418-z