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Underground hydrogen storage has been recognized as a key technology for storing enormous amounts of hydrogen, thus aiding in the industrial-scale application of a hydrogen economy. However, underground hydrogen storage is only poorly understood, which leads to high project risk. This research thus examined the effect of caprock availability and hydrogen injection rate on hydrogen recovery factor and hydrogen leakage rate to address some fundamental questions related to underground hydrogen storage. A three dimensional heterogeneous reservoir model was developed, and the impact of caprock and hydrogen injected rate on hydrogen underground storage efficiency were analysed with the model. The results indicate that both caprock and injection rate have an important impact on hydrogen leakage, and the quantities of trapped and recovered hydrogen. It is concluded that higher injection rate increases H 2 leakage when caprocks are absent. In addition, lower injection rates and caprock availability increases the amount of recovered hydrogen. This work therefore provided fundamental information regarding underground hydrogen storage project assessment, and supports the decarbonisation of the energy supply chain.


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Hydrogen underground storage efficiency in a heterogeneous sandstone reservoir

Show Author's information Doaa Saleh Mahdi1Emad A. Al-Khdheeawi1,2Yujie Yuan3,4Yihuai Zhang5Stefan Iglauer6
Petroleum Technology Department, University of Technology, Baghdad 10066, Iraq
Western Australia School of Mines: Minerals, Energy and Chemical Engineering, Discipline of Petroleum Engineering, Curtin University, Kensington 6151, Western Australia, Australia
School of Earth Sciences, Yunnan University, Kunming 650500, P. R. China
Key Laboratory of Deep-Earth Dynamics of Ministry of Natural Resources, Chinese Academy of Geological Sciences, Institute of Geology, Beijing 100037, P. R. China
Department of Earth Science and Engineering, Imperial College London, London SW7 2BP, UK
School of Engineering, Edith Cowan University, Joondalup 6027, Western Australia, Australia

Abstract

Underground hydrogen storage has been recognized as a key technology for storing enormous amounts of hydrogen, thus aiding in the industrial-scale application of a hydrogen economy. However, underground hydrogen storage is only poorly understood, which leads to high project risk. This research thus examined the effect of caprock availability and hydrogen injection rate on hydrogen recovery factor and hydrogen leakage rate to address some fundamental questions related to underground hydrogen storage. A three dimensional heterogeneous reservoir model was developed, and the impact of caprock and hydrogen injected rate on hydrogen underground storage efficiency were analysed with the model. The results indicate that both caprock and injection rate have an important impact on hydrogen leakage, and the quantities of trapped and recovered hydrogen. It is concluded that higher injection rate increases H 2 leakage when caprocks are absent. In addition, lower injection rates and caprock availability increases the amount of recovered hydrogen. This work therefore provided fundamental information regarding underground hydrogen storage project assessment, and supports the decarbonisation of the energy supply chain.

Keywords: Hydrogen storage, reservoir simulation, hydrogen recovery, heterogeneous reservoirs, hydrogen leakage

References(42)

Acar, C., Dincer, I. Review and evaluation of hydrogen production options for better environment. Journal of Cleaner Production, 2019, 218: 835-849.
Al-Khdheeawi, E. A., Vialle, S., Barifcani, A., et al. Impact of reservoir wettability and heterogeneity on CO2-plume migration and trapping capacity. International Journal of Greenhouse Gas Control, 2017a, 58: 142-158.
Al-Khdheeawi, E. A., Vialle, S., Barifcani, A., et al. Influence of CO2-wettability on CO2 migration and trapping capacity in deep saline aquifers. Greenhouse Gases: Science and Technology, 2017b, 7(2): 328-338.
Al-Khdheeawi, E. A., Vialle, S., Barifcani, A., et al. Influence of injection well configuration and rock wettability on CO2 plume behaviour and CO2 trapping capacity in heterogeneous reservoirs. Journal of Natural Gas Science and Engineering, 2017c, 43: 190-206.
Al-Khdheeawi, E. A., Vialle, S., Barifcani, A., et al. Enhancement of CO2 trapping efficiency in heterogeneous reservoirs by water-alternating gas injection. Greenhouse Gases: Science and Technology, 2018, 8(5): 920-931.
Ali, M., Yekeen, N., Pal, N., et al. Influence of pressure, temperature and organic surface concentration on hydrogen wettability of caprock; implications for hydrogen geo-storage. Energy Reports, 2021, 7: 5988-5996.
Bai, M., Song, K., Sun, Y., et al. An overview of hydrogen underground storage technology and prospects in China. Journal of Petroleum Science and Engineering, 2014, 124: 132-136.
Basniev, K. S., Omelchenko, R. J., Adzynova, F. A. Underground hydrogen storage problems in Russia. Paper Presented at 18th World Hydrogen Energy Conference 2010-WHEC 2010, Essen, Germany, 16-21 May, 2010.
Battistelli, A., Calore, C., Pruess, K. The simulator TOUGH2/EWASG for modelling geothermal reservoirs with brines and non-condensible gas. Geothermics, 1997, 26(4): 437-464.
Berta, M., Dethlefsen, F., Ebert, M., et al. Geochemical effects of millimolar hydrogen concentrations in groundwater: An experimental study in the context of subsurface hydrogen storage. Environmental Science and Technology, 2018, 52(8): 4937-4949.
Crotogino, F., Donadei, S., Bünger, U., et al. Large-scale hydrogen underground storage for securing future energy supplies. Paper Presented at 18th World Hydrogen Energy Conference 2010-WHEC 2010, Essen, Germany, 16-21 May, 2010.
Dake, L. P. Fundamentals of Reservoir Engineering. Amsterdam, the Netherlands, Elsevier Science, 1978.
Fossen, H. Structural Geology. Cambridge, UK, Cambridge University Press, 2016.
DOI
Han, G., Kwon, Y. K., Kim, J. B., et al. Development of a high-energy-density portable/mobile hydrogen energy storage system incorporating an electrolyzer, a metal hydride and a fuel cell. Applied Energy, 2020, 259: 114175.
Hanley, E. S., Deane, J. P., Gallachóir, B. P. Ó. The role of hydrogen in low carbon energy futures-A review of existing perspectives. Renewable and Sustainable Energy Reviews, 2018, 82: 3027-3045.
Iglauer, S., Ali, M., Keshavarz, A. Hydrogen wettability of sandstone reservoirs: Implications for hydrogen geo-storage. Geophysical Research Letters, 2021, 48(3): e2020GL090814.
Iglauer, S., Al-Yaseri, A. Improving basalt wettability to de-risk CO2 geo-storage in basaltic formations. Advances in Geo-Energy Research, 2021, 5(3): 347-350.
International Energy Agency (2020) World Energy Outlook.
Leverett, M. Capillary behavior in porous solids. Transactions of the AIME, 1941, 142(1): 152-169.
Lord, A. S., Kobos, P. H., Borns, D. J. Geologic storage of hydrogen: Scaling up to meet city transportation demands. International Journal of Hydrogen Energy, 2014, 39(28): 15570-15582.
Luboń, K., Tarkowski, R. Numerical simulation of hydrogen injection and withdrawal to and from a deep aquifer in NW Poland. International Journal of Hydrogen Energy, 2020, 45(3): 2068-2083.
Matos, C. R., Carneiro, J. F., Silva, P. P. Overview of large-scale underground energy storage technologies for integration of renewable energies and criteria for reservoir identification. Journal of Energy Storage, 2019, 21: 241-258.
Metz, B., Davidson, O., De Coninck, H. C., et al. Ipcc Special Report on Carbon Dioxide Capture and Storage. Cambridge, UK, Cambridge University Press, 2005.
Mualem, Y. A new model for predicting the hydraulic conductivity of unsaturated porous media. Water Resources Research, 1976, 12(3): 513-522.
Ni, M., Leung, M. K. H., Sumathy, K., et al. Potential of renewable hydrogen production for energy supply in Hong Kong. International Journal of Hydrogen Energy, 2006, 31(10): 1401-1412.
Ozarslan, A. Large-scale hydrogen energy storage in salt caverns. International Journal of Hydrogen Energy, 2012, 37(19): 14265-14277.
Pan, B., Yin, X., Ju, Y., et al. Underground hydrogen storage: Influencing parameters and future outlook. Advances in Colloid and Interface Science, 2021, 294: 102473.
Panfilov, M. Underground and pipeline hydrogen storage, in Compendium of Hydrogen Energy, Volume 2: Hydrogen Storage, Distribution and Infrastructure, edited by R. B. Gupta, A. Basile and T. N. Veziroğlu, Woodhead Publishing, Cambridge, pp. 91-115, 2016.
DOI
Paterson, L. The implications of fingering in underground hydrogen storage. International Journal of Hydrogen Energy, 1983, 8(1): 53-59.
Pruess, K., Oldenburg, C., Moridis, G. TOUGH2 User’s Guide Version 2. Lawrence Berkeley National Laboratory, 1999.
Seo, S. K., Yun, D. Y., Lee, C. J. Design and optimization of a hydrogen supply chain using a centralized storage model. Applied Energy, 2020, 262: 114452.
Song, Y. New perspectives on potential hydrogen storage materials using high pressure. Physical Chemistry Chemical Physics, 2013, 15(35): 14524-14547.
Stalker, L., Varma, S., Van Gent, D., et al. South eest hub: A carbon capture and storage project. Australian Journal of Earth Sciences, 2013, 60(1): 45-58.
Tarkowski, R. Underground hydrogen storage: Characteristics and prospects. Renewable and Sustainable Energy Reviews, 2019, 105: 86-94.
Tiab, D., Donaldson, E. C. Petrophysics. Amsterdam, the Netherlands, Elsevier, 2004.
Tian, H., Xu, T., Li, Y., et al. Evolution of sealing efficiency for CO2 geological storage due to mineral alteration within a hydrogeologically heterogeneous caprock. Applied Geochemistry, 2015, 63: 380-397.
Van Genuchten, M. T. A closed-form equation for predicting the hydraulic conductivity of unsaturated soils. Soil Science Society of America Journal, 1980, 44(5): 892-898.
Yartys, V. A., Lototsky, M. V. An overview of hydrogen storage methods, in Hydrogen Materials Science and Chemistry of Carbon Nanomaterials, edited by T. Nejat Veziroglu, Svetlana Yu. Zaginaichenko, Dmitry V. Schur, B. Baranowski, Anatoliy P. Shpak, Valeriy V. Skorokhod, Springer, Dordrecht, pp. 75-104, 2004.
Yekta, A., Pichavant, M., Audigane, P. Evaluation of geochemcial reactivity of hydrogen in sandstone: Application to geoogic stoage. Applied Geochemistry, 2018a, 95: 182-194.
Yekta, A. E., Manceau, J. C., Gaboreau, S., et al. Determination of hydrogen-water relative permeability and capillary pressure in sandstone: Application to underground hydrogen injection in sedimentary formations. Transport in Porous Media, 2018b, 122(2): 333-356.
Zhang, F., Zhao, P., Niu, M., et al. The survey of key technologies in hydrogen energy storage. International Journal of Hydrogen Energy, 2016, 41(33): 14535-14552.
Zivar, D., Kumar, S., Foroozesh, J. Underground hydrogen storage: A comprehensive review. International Journal of Hydrogen Energy, 2021, 46(45): 23436-23462.
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Publication history

Received: 06 November 2021
Revised: 18 November 2021
Accepted: 19 November 2021
Published: 21 November 2021
Issue date: December 2021

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© The Author(s) 2021.

Acknowledgements

Emad A. Al-Khdheeawi and Doaa S. Mahdi appreciates the University of Technology for the support. Yujie Yuan would like to thank the funding from the Key Laboratory of Deep-Earth Dynamics of Ministry of Natural Resources (Funding Number: J1901), Institute of Geology, Chinese Academy of Geological Sciences, Beijing.

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This article is distributed under the terms and conditions of the Creative Commons Attribution (CC BY-NC-ND) license, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.

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