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Research Article | Open Access

Building the conformal protection of VB-group VS2 laminated heterostructure based on biomass-derived carbon for excellent broadband electromagnetic waves absorption

Honghan Wanga,b, Huibin Zhanga, Junye Chengc( ), Tingting Liud, Deqing Zhanga( ), Guangping Zhenge, Shangru Zhaib( ), Maosheng Caod( )
School of Materials Science and Engineering, Qiqihar University, Qiqihar, 161006, China
Liaoning Key Lab of Lignocellulose Chemistry and BioMaterials, Liaoning Collaborative Innovation Center for Lignocellulosic Biorefinery, College of Light Industry and Chemical Engineering, Dalian Polytechnic University, Dalian, 116034, China
Department of Materials Science, Shenzhen MSU-BIT University, Shenzhen, Guangdong Province, 517182, China
School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, 100081, China
Department of Mechanical Engineering, Hong Kong Polytechnic University, Hung Hom, Kowloon, Hong Kong, China

Peer review under responsibility of The Chinese Ceramic Society.

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Graphical Abstract

Abstract

Although VB-Group transition metal disulfides (TMDs) VS2 nanomaterials with specific electronic properties and multiphase microstructures have shown fascinating potential in the field of electromagnetic wave (EMW) absorption, the efficient utilization of VS2 is limited by the technical bottleneck of its narrow effective absorption bandwidth (EAB) which is attributed to environmental instability and a deficient electromagnetic (EM) loss mechanism. In order to fully exploit the maximal utilization values of VS2 nanomaterials for EMW absorption through mitigating the chemical instability and optimizing the EM parameters, biomass-based glucose derived carbon (GDC) like sugar-coating has been decorated on the surface of stacked VS2 nanosheets via a facile hydrothermal method, followed by high-temperature carbonization. As a result, the modulation of doping amount of glucose injection solution (Glucose) could effectively manipulate the encapsulation degree of GDC coating on VS2 nanosheets, further implementing the EM response mechanisms of the VS2/GDC hybrids (coupling effect of conductive loss, interfacial polarization, relaxation, dipole polarization, defect engineering and multiple reflections and absorptions) through regulating the conductivity and constructing multi-interface heterostructures, as reflected by the enhanced EMW absorption performance to a great extent. The minimum reflection loss (Rmin) of VS2/GDC hybrids could reach −52.8 dB with a thickness of 2.7 mm at 12.2 GHz. Surprisingly, compared with pristine VS2, the EAB of the VS2/GDC hybrids increased from 2.0 to 5.7 GHz, while their environmental stability was effectively enhanced by virtue of GDC doping. Obviously, this work provides a promising candidate to realize frequency band tunability of EMW absorbers with exceptional performance and environmental stability.

Keywords

VS2/GDC hybridsMulti-interface heterostructuresBroadband absorptionEnvironmental stability

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Journal of Materiomics
Volume 9 Issue 3,
May 2023
Pages 492-501
DOI: 10.1016/j.jmat.2022.12.003
Cite this article:
Wang H, Zhang H, Cheng J, et al. Building the conformal protection of VB-group VS2 laminated heterostructure based on biomass-derived carbon for excellent broadband electromagnetic waves absorption. Journal of Materiomics, 2023, 9(3): 492-501. https://doi.org/10.1016/j.jmat.2022.12.003

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Received: 09 October 2022
Revised: 28 November 2022
Accepted: 10 December 2022
Published: 19 January 2023
© 2023 The Authors.

This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
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