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Research paper | Open Access

Phase transition and piezoelectric property of (Ag, K)NbO3 ceramics

Lin Chena,b,1Mingyuan Zhaoa,1Jing Wangb( )Suwei ZhangcFuhua SundLei Zhaoa( )
Key Laboratory of High-precision Computation and Application of Quantum Field Theory of Hebei Province, College Physics Science and Technology, Hebei University, Baoding, 071002, China
Key Laboratory of Mechanics and Control of Mechanical Structures, College of Aerospace Engineering, Nanjing University of Aeronautics and Astronautics, Nanjing, 210016, China
Center for Advanced Measurement Science, National Institute of Metrology, Beijing, 100029, China
Institute for Advanced Materials, Hubei Normal University, Huangshi, 435002, China

Peer review under responsibility of The Chinese Ceramic Society.

1 These authors contributed equally.

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Graphical Abstract

Abstract

AgNbO3 is an antiferroelectric (AFE) material with double hysteresis loop. Both the antiferroelectricity and ferroelectricity can be enhanced by doping. Herein, the ferroelectricity of AgNbO3 ceramics was enhanced via K-doping and the phase diagram of the (Ag1-xKx)NbO3 ceramics was upgraded. In details, (Ag1-xKx)NbO3 ceramics are ferrielectric (FIE) M1 phase as x = 5.00–5.50 mol% and ferroelectric (FE) O phase as x = 5.75–6.00 mol% before poling, and FE O phase as x = 5.00–6.00 mol% after poling at room temperature. With increasing temperature, (Ag1-xKx)NbO3 ceramics show the phase evolutions from FIE M1, AFE M2 to paraelectric (PE) T phase at x = 5.00–5.50 mol% and from FE O, FE T to PE T phase at x = 5.75–6.00 mol% before poling, and from FE O, FE T to PE T phase at x = 5.00–6.00 mol% after poling. High d33 values of 180 pC/N and 285 pC/N are obtained at the FE O-FE T and FE T-PE T phase boundaries. This work sheds light on a novel and promising lead-free piezoelectric system.

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Journal of Materiomics
Pages 863-872
Cite this article:
Chen L, Zhao M, Wang J, et al. Phase transition and piezoelectric property of (Ag, K)NbO3 ceramics. Journal of Materiomics, 2022, 8(4): 863-872. https://doi.org/10.1016/j.jmat.2022.01.001

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Received: 15 November 2021
Revised: 21 December 2021
Accepted: 02 January 2022
Published: 05 January 2022
© 2022 The Chinese Ceramic Society.

This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).

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