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Full Length Article | Open Access

Machine learning-guided accelerated discovery of structure-property correlations in lean magnesium alloys for biomedical applications

Sreenivas Raguramana,b( ), Maitreyee Sharma Priyadarshinic, Tram Nguyena,d, Ryan McGoverne, Andrew Kima, Adam J. Griebelf, Paulette Clancyb,c, Timothy P. Weihsa,b,g( )
Department of Materials Science and Engineering, Johns Hopkins University, 3400 N Charles St, Baltimore, 21218, MD, U.S.A
Hopkins Extreme Materials Institute, Johns Hopkins University, 3400 N Charles St, Baltimore, 21218, MD, U.S.A
Department of Chemical and Biomolecular Engineering, Johns Hopkins University, 3400 N Charles St, Baltimore, 21218, MD, U.S.A
Translational Tissue Engineering Center, Johns Hopkins School of Medicine, 400 N Broadway, Baltimore, 21231, MD, U.S.A
Department of Biomedical Engineering, Johns Hopkins University, 3400 N Charles St, Baltimore, 21218, MD, U.S.A
Research and Development, Fort Wayne Metals Research Products, LLC, 9609 Ardmore Ave, Fort Wayne, 46809, IN, U.S.A
Department of Mechanical Engineering, Johns Hopkins University, 3400 N Charles St, Baltimore, 21218, MD, U.S.A
Show Author Information

Abstract

Magnesium alloys are emerging as promising alternatives to traditional orthopedic implant materials thanks to their biodegradability, biocompatibility, and impressive mechanical characteristics. However, their rapid in-vivo degradation presents challenges, notably in upholding mechanical integrity over time. This study investigates the impact of high-temperature thermal processing on the mechanical and degradation attributes of a lean Mg-Zn-Ca-Mn alloy, ZX10. Utilizing rapid, cost-efficient characterization methods like X-ray diffraction and optical microscopy, we swiftly examine microstructural changes post-thermal treatment. Employing Pearson correlation coefficient analysis, we unveil the relationship between microstructural properties and critical targets (properties): hardness and corrosion resistance. Additionally, leveraging the least absolute shrinkage and selection operator (LASSO), we pinpoint the dominant microstructural factors among closely correlated variables. Our findings underscore the significant role of grain size refinement in strengthening and the predominance of the ternary Ca2Mg6Zn3 phase in corrosion behavior. This suggests that achieving an optimal blend of strength and corrosion resistance is attainable through fine grains and reduced concentration of ternary phases. This thorough investigation furnishes valuable insights into the intricate interplay of processing, structure, and properties in magnesium alloys, thereby advancing the development of superior biodegradable implant materials.

Keywords

Magnesium alloysMachine learningCorrosionMechanical propertiesRapid characterization

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Journal of Magnesium and Alloys
Volume 12 Issue 6,
June 2024
Pages 2267-2283
DOI: 10.1016/j.jma.2024.06.008
Cite this article:
Raguraman S, Priyadarshini MS, Nguyen T, et al. Machine learning-guided accelerated discovery of structure-property correlations in lean magnesium alloys for biomedical applications. Journal of Magnesium and Alloys, 2024, 12(6): 2267-2283. https://doi.org/10.1016/j.jma.2024.06.008

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Received: 19 April 2024
Revised: 08 June 2024
Accepted: 12 June 2024
Published: 28 June 2024
© 2024 Chongqing University.

This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/) Peer review under responsibility of Chongqing University
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